作者
JA De Jong, I Razdolski, AM Kalashnikova, RV Pisarev, AM Balbashov, Andrei Kirilyuk, Th Rasing, AV Kimel
发表日期
2012/4/13
期刊
Physical Review Letters
卷号
108
期号
15
页码范围
157601
出版商
American Physical Society
简介
Time-resolved magneto-optical imaging of laser-excited rare-earth orthoferrite demonstrates that a single 60 fs circularly polarized laser pulse is capable of creating a magnetic domain on a picosecond time scale with a magnetization direction determined by the helicity of light. Depending on the light intensity and sample temperature, pulses of the same helicity can create domains with opposite magnetizations. We argue that this phenomenon relies on a twofold effect of light which (i) instantaneously excites coherent low-amplitude spin precession and (ii) triggers a spin reorientation phase transition. The former dynamically breaks the equivalence between two otherwise degenerate states with opposite magnetizations in the high-temperature phase and thus controls the route of the phase transition.
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