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High-potassium felsic volcanic rocks interlayered with basalt and komatiite in early Archaean greenstone sequences in the Barberton Greenstone Belt of South Africa and Swaziland, previously considered to be derived from melting of mafic precursors, are shown to be the result of melting of significantly older felsic crust. This is documented by a combination of SHRIMP zircon dating with Hf-in-zircon and whole-rock Lu–Hf and Sm–Nd isotopic data. Zircons from felsic rocks of the oldest Barberton unit, the 3.53 Ga Theespruit Formation, yielded predominantly negative ε Hf (t)-values, whereas whole-rock ε Hf (t)-and ε Nd (t)-data are slightly negative to slightly positive. Similar results were obtained for ca. 3.45 Ga felsic rocks in the Hoeggenoog and Noisy Formations higher up in the greenstone stratigraphy. These data rule out derivation of the felsic units from melting of basaltic precursors and favor a crustal source …