作者
Roseline Cutting Thakur, Lubna Dada, Lisa J Beck, Lauriane LJ Quéléver, Tommy Chan, Marjan Marbouti, Xu-Cheng He, Carlton Xavier, Juha Sulo, Janne Lampilahti, Markus Lampimäki, Yee Jun Tham, Nina Sarnela, Katrianne Lehtipalo, Alf Norkko, Markku Kulmala, Mikko Sipilä, Tuija Jokinen
发表日期
2021/10/4
期刊
Atmospheric Chemistry and Physics Discussions
卷号
2021
页码范围
1-45
简介
Several studies have investigated New Particle Formation (NPF) events from various sites ranging from pristine locations, including (boreal) forest sites to urban areas. However, there is still a dearth of studies investigating NPF processes and subsequent aerosol growth in coastal yet semi-urban sites, where the tropospheric layer is a concoction of biogenic and anthropogenic gases and particles. The investigation of factors leading to NPF becomes extremely complex due to the highly dynamic meteorological conditions at the coastline especially when combined with both continental and oceanic weather conditions. Herein, we engage a comprehensive study of particle number size distributions and aerosol-forming precursor vapors at the coastal semi-urban site in Helsinki, Finland. The measurement period, 25 June 2019–18 August 2019, was timed with the recurring cyanobacterial summer bloom in the Baltic Sea region and coastal regions of Finland. Our study recorded several regional/local NPF and aerosol burst events during this period. Although the overall anthropogenic influence on Sulfuric Acid (SA) concentrations was low during the measurement period, we observed that the regional or local NPF events, characterized by SA concentrations in the order of 107 molecules per cm−3 occurred mostly when the air mass travelled over the land areas. Interestingly, when the air mass travelled over the Baltic Sea, an area enriched with Algae and cyanobacterial blooms, high Iodic Acid (IA) concentration coincided with an aerosol burst or a spike event at the measurement site. Further, SA-rich bursts were seen when the air mass travelled …
引用总数
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