作者
Helen M Amos, Daniel J Jacob, David Kocman, Hannah M Horowitz, Yanxu Zhang, Stephanie Dutkiewicz, Milena Horvat, Elizabeth S Corbitt, David P Krabbenhoft, Elsie M Sunderland
发表日期
2014/8/19
期刊
Environmental science & technology
卷号
48
期号
16
页码范围
9514-9522
出版商
American Chemical Society
简介
Rivers are an important source of mercury (Hg) to marine ecosystems. Based on an analysis of compiled observations, we estimate global present-day Hg discharges from rivers to ocean margins are 27 ± 13 Mmol a–1 (5500 ± 2700 Mg a–1), of which 28% reaches the open ocean and the rest is deposited to ocean margin sediments. Globally, the source of Hg to the open ocean from rivers amounts to 30% of atmospheric inputs. This is larger than previously estimated due to accounting for elevated concentrations in Asian rivers and variability in offshore transport across different types of estuaries. Riverine inputs of Hg to the North Atlantic have decreased several-fold since the 1970s while inputs to the North Pacific have increased. These trends have large effects on Hg concentrations at ocean margins but are too small in the open ocean to explain observed declines of seawater concentrations in the North Atlantic …
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