作者
Miriam Varón, Marco Beleggia, Takeshi Kasama, RJ Harrison, Rafal E Dunin-Borkowski, Víctor F Puntes, Cathrine Frandsen
发表日期
2013/2/6
期刊
Scientific reports
卷号
3
期号
1
页码范围
1234
出版商
Nature Publishing Group UK
简介
Magnetostatic (dipolar) interactions between nanoparticles promise to open new ways to design nanocrystalline magnetic materials and devices if the collective magnetic properties can be controlled at the nanoparticle level. Magnetic dipolar interactions are sufficiently strong to sustain magnetic order at ambient temperature in assemblies of closely-spaced nanoparticles with magnetic moments of ≥ 100 μB. Here we use electron holography with sub-particle resolution to reveal the correlation between particle arrangement and magnetic order in self-assembled 1D and quasi-2D arrangements of 15 nm cobalt nanoparticles. In the initial states, we observe dipolar ferromagnetism, antiferromagnetism and local flux closure, depending on the particle arrangement. Surprisingly, after magnetic saturation, measurements and numerical simulations show that overall ferromagnetic order exists in the present nanoparticle …
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