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Ecofriendly, highly effective, and low-cost solar steam generation has great potential in the applications of power generation, seawater desalination, and industry wastewater treatment. Solar steam generation requires an evaporator that has strong light absorption over a wide-frequency band (200–3000 nm), high photothermal conversion efficiency, and good thermal insulation to avoid excessive heat loss. Herein, foam-strengthened ultrablack carbon aerogels (CAs) with micropores, mesopores, and macropores were prepared using freeze drying. The small-size conductor effect in ultrablack CAs could increase the surface electron concentration, leading to the increase of light absorption and ultimately enhancing photothermal conversion efficiency. Consequently, under 1 sun illumination, dried CA-5 exhibited a fast temperature rise rate and the highest thermal equilibrium temperature of 87.6 °C among CAs, the …