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Novel design of flexible chiral metasurface has been attractive to control electromagnetic dynamics for fabricating integrated enantiomeric sensing devices. In this article, a reconfigurable metasurface decorated with planar magnetoplasmonic microbundle arrays of Au@Fe₃O₄ core‐shell nanowires (NWs) on polydimethylsiloxane film is fabricated. Its chiroptical property is willingly manipulated by skew angle (θ), that is, the angle between applied magnetic field vector (B) and tangent vector (T) of a curved metasurface. Interestingly, the as‐prepared NW metasurface presents many internal skew angles (θ_in) among respective NWs at nanoscale as well as additional external skew angle (θ_ex) among arrays at microscale, extraordinarily enhancing chiroptical signal compared to other nanosphere or single NW arrays where lack of θ_in is observed. Computational simulation proves the disruption of the symmetry via …