作者
Guichuan Xing, Nripan Mathews, Swee Sien Lim, Natalia Yantara, Xinfeng Liu, Dharani Sabba, Michael Grätzel, Subodh Mhaisalkar, Tze Chien Sum
发表日期
2014/5
期刊
Nature materials
卷号
13
期号
5
页码范围
476-480
出版商
Nature Publishing Group UK
简介
Low-temperature solution-processed materials that show optical gain and can be embedded into a wide range of cavity resonators are attractive for the realization of on-chip coherent light sources. Organic semiconductors and colloidal quantum dots are considered the main candidates for this application. However, stumbling blocks in organic lasing,,, include intrinsic losses from bimolecular annihilation and the conflicting requirements of high charge carrier mobility and large stimulated emission; whereas challenges pertaining to Auger losses and charge transport in quantum dots,, still remain. Herein, we reveal that solution-processed organic–inorganic halide perovskites (CH3NH3PbX3 where X = Cl, Br, I), which demonstrated huge potential in photovoltaics,,,, also have promising optical gain. Their ultra-stable amplified spontaneous emission at strikingly low thresholds stems from their large absorption …
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