作者
Mingjian Yuan, Li Na Quan, Riccardo Comin, Grant Walters, Randy Sabatini, Oleksandr Voznyy, Sjoerd Hoogland, Yongbiao Zhao, Eric M Beauregard, Pongsakorn Kanjanaboos, Zhenghong Lu, Dong Ha Kim, Edward H Sargent
发表日期
2016/10
期刊
Nature nanotechnology
卷号
11
期号
10
页码范围
872-877
出版商
Nature Publishing Group UK
简介
Organometal halide perovskites exhibit large bulk crystal domain sizes, rare traps, excellent mobilities and carriers that are free at room temperature—properties that support their excellent performance in charge-separating devices. In devices that rely on the forward injection of electrons and holes, such as light-emitting diodes (LEDs), excellent mobilities contribute to the efficient capture of non-equilibrium charge carriers by rare non-radiative centres. Moreover, the lack of bound excitons weakens the competition of desired radiative (over undesired non-radiative) recombination. Here we report a perovskite mixed material comprising a series of differently quantum-size-tuned grains that funnels photoexcitations to the lowest-bandgap light-emitter in the mixture. The materials function as charge carrier concentrators, ensuring that radiative recombination successfully outcompetes trapping and hence non-radiative …
引用总数
20162017201820192020202120222023202414150280313340360293241104
学术搜索中的文章
M Yuan, LN Quan, R Comin, G Walters, R Sabatini… - Nature nanotechnology, 2016