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The esthetic clasp material is a clinical demand for a satisfactory removable partial denture. The purpose of this study is to assess the mechanical performance of graphene-based polymer (GBP) and polyether-ether-ketone (PEEK) materials as clasp materials. Thirty-two clasps were fabricated by CAD-CAM from two materials, GBP and PEEK. All clasps were tested for retention force after 10,000 cycles of insertion and removal and thermocycling. The clasp arms’ deformation was measured, and areas of stress–strain concentration were explored. The Mann–Whitney U test was used to compare the retentive force of the studied groups, while the independent sample t-test was applied to check the difference in clasp arm deformation at α = 0.5. The results showed a significantly higher retentive force (2.248 ± 0.315 N) in PEEK clasps, at p < 0.001. The deformation of the clasp arm of the GBP clasps was significantly higher than PEEK clasps. Areas of stress–strain concentration were seen at the junction of the retentive arm to the minor connector and at the retentive arm terminal. It could be concluded that PEEK polymer had a better mechanical performance as an esthetic clasp material than the GBP. An optimization study for GBP might be required to check the validity of such an application.