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This study aimed at investigating optimal experience during schoolwork in relation to SDT concepts of autonomy and locus of causality. Data were gathered from 268 high-school students using Experience Sampling Method for 1 week. Three levels of self-determination were identified: high (corresponding to autonomous regulation), moderate (mixed autonomous and controlled regulation), and low (controlled regulation). Consistently with the literature, the relationship between participants’ challenges and skills values was used to recognize occasions for optimal experience, and multilevel modeling was applied in data analysis. Findings showed that during schoolwork as optimal activity (high challenges and high skills) students mostly reported low levels of self-determination. However, the quality of their experience was better in situations of high and moderate self-determination. At the theoretical level …