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The transformation processes of hexachlorocyclohexane isomers (HCHs) from production sites of Lindane across the landscape and along the food web were studied as an example to understand the fate of POPs in the environment. Therefore, we studied the concentration and isotope composition of HCHs in different matrices in the vicinity of a dumpsite and a chemical plant producing HCHs in India. Carbon isotope compositions (δ¹³C) of HCHs and the enantiomer fraction (EF) of α-HCH were used as indicators to characterize in situ degradation in soil, groundwater, and sediment as well as along the food web. The HCHs were detected in plants growing on contaminated soil. Elevated concentrations of HCHs were found in a number of crops, which indicates an important transfer pathway of HCHs entering food webs. The EF value of α-HCH and the δ¹³C signature of HCHs indicated that degradation processes …