作者
Dominik Stolzenburg, Lukas Fischer, Alexander L Vogel, Martin Heinritzi, Meredith Schervish, Mario Simon, Andrea C Wagner, Lubna Dada, Lauri R Ahonen, Antonio Amorim, Andrea Baccarini, Paulus S Bauer, Bernhard Baumgartner, Anton Bergen, Federico Bianchi, Martin Breitenlechner, Sophia Brilke, Stephany Buenrostro Mazon, Dexian Chen, António Dias, Danielle C Draper, Jonathan Duplissy, Imad El Haddad, Henning Finkenzeller, Carla Frege, Claudia Fuchs, Olga Garmash, Hamish Gordon, Xucheng He, Johanna Helm, Victoria Hofbauer, Christopher R Hoyle, Changhyuk Kim, Jasper Kirkby, Jenni Kontkanen, Andreas Kürten, Janne Lampilahti, Michael Lawler, Katrianne Lehtipalo, Markus Leiminger, Huajun Mai, Serge Mathot, Bernhard Mentler, Ugo Molteni, Wei Nie, Tuomo Nieminen, John B Nowak, Andrea Ojdanic, Antti Onnela, Monica Passananti, Tuukka Petäjä, Lauriane LJ Quéléver, Matti P Rissanen, Nina Sarnela, Simon Schallhart, Christian Tauber, António Tomé, Robert Wagner, Mingyi Wang, Lena Weitz, Daniela Wimmer, Mao Xiao, Chao Yan, Penglin Ye, Qiaozhi Zha, Urs Baltensperger, Joachim Curtius, Josef Dommen, Richard C Flagan, Markku Kulmala, James N Smith, Douglas R Worsnop, Armin Hansel, Neil M Donahue, Paul M Winkler
发表日期
2018/9/11
期刊
Proceedings of the National Academy of Sciences
卷号
115
期号
37
页码范围
9122-9127
出版商
National Academy of Sciences
简介
Nucleation and growth of aerosol particles from atmospheric vapors constitutes a major source of global cloud condensation nuclei (CCN). The fraction of newly formed particles that reaches CCN sizes is highly sensitive to particle growth rates, especially for particle sizes 10 nm, where coagulation losses to larger aerosol particles are greatest. Recent results show that some oxidation products from biogenic volatile organic compounds are major contributors to particle formation and initial growth. However, whether oxidized organics contribute to particle growth over the broad span of tropospheric temperatures remains an open question, and quantitative mass balance for organic growth has yet to be demonstrated at any temperature. Here, in experiments performed under atmospheric conditions in the Cosmics Leaving Outdoor Droplets (CLOUD) chamber at the European Organization for Nuclear Research (CERN), we …
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D Stolzenburg, L Fischer, AL Vogel, M Heinritzi… - Proceedings of the National Academy of Sciences, 2018