作者
Abraham Dearden, Yicong He, Ali Akherati, Christopher Lim, Matthew Coggon, Abigail Koss, Joost de Gouw, Carsten Warneke, Lindsay Yee, John H Seinfeld, Christopher Cappa, Jesse H Kroll, Jeffrey R Pierce, Shantanu Jathar
发表日期
2024
期刊
Environmental Science: Atmospheres
出版商
Royal Society of Chemistry
简介
Biomass burning is an important source of primary and secondary organic aerosol (POA, SOA, and together, OA) to the atmosphere. The photochemical evolution of biomass burning OA, especially over long photochemical ages, is highly complex and there are large uncertainties in how this evolution is represented in models. Recently, Lim et al. (2019) performed and reported on photooxidation experiments of biomass burning emissions using a small environmental chamber (~150 L) to study the OA evolution over multiple equivalent days of photochemical aging. In this work, we use a kinetic, process-level model (SOM-TOMAS; Statistical Oxidation Model-TwO Moment Aerosol Sectional) to simulate the photochemical evolution of OA in 18 chamber experiments performed on emissions from 10 different fuels. A base version of the model was able to simulate the time-dependent evolution of the OA mass …
学术搜索中的文章
A Dearden, Y He, A Akherati, C Lim, M Coggon, A Koss… - Environmental Science: Atmospheres, 2024