作者
Catalin D Spataru, Sohrab Ismail-Beigi, Rodrigo B Capaz, Steven G Louie
发表日期
2005/12/9
期刊
Physical review letters
卷号
95
期号
24
页码范围
247402
出版商
American Physical Society
简介
We present a theoretical analysis and first-principles calculation of the radiative lifetime of excitons in semiconducting carbon nanotubes. An intrinsic lifetime of the order of 10 ps is computed for the lowest optically active bright excitons. The intrinsic lifetime is, however, a rapid increasing function of the exciton momentum. Moreover, the electronic structure of the nanotubes dictates the existence of dark excitons near in energy to each bright exciton. Both effects strongly influence measured lifetime. Assuming a thermal occupation of bright and dark exciton bands, we find an effective lifetime of the order of 10 ns at room temperature, in good accord with recent experiments.
引用总数
20062007200820092010201120122013201420152016201720182019202020212022202320243233372521382825201711202328121917179