作者
Karn Vohra, Eloise Marais, Gongda Lu, William Bloss, Lei Zhu, Henk Eskes, Isabelle De Smedt
发表日期
2021/1/18
期刊
Earth and Space Science Open Archive ESSOAr
出版商
American Geophysical Union
简介
Policies to regulate severe surface ozone pollution in cities in India are challenging to develop, due to the complex dependence on precursor emissions of volatile organic compounds (VOCs) and nitrogen oxides (NOx), non-linear chemistry leading to ozone formation, and very limited spatial and temporal surface air quality monitoring. Ratios of space-based observations of formaldehyde (HCHO), an intermediate oxidation product of VOCs, and nitrogen dioxide (NO2) have been used to characterize the sensitivity of surface ozone production to precursor emissions of VOCs and NOx, but interpretation of these depends on the local oxidation regime. Here we develop an improved approach in which we discretize the data into background HCHO due to methane and other long-lived VOCs (regression intercept) and the local relationship (regression slope) between HCHO associated with reactive VOCs and NO2. We …
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K Vohra, E Marais, G Lu, W Bloss, L Zhu, H Eskes… - Earth and Space Science Open Archive ESSOAr, 2021