作者
Sangyong Lee, Liyuan Liang, David Riestenberg, Olivia R West, Costas Tsouris, Eric Adams
发表日期
2003/8/15
期刊
Environmental science & technology
卷号
37
期号
16
页码范围
3701-3708
出版商
American Chemical Society
简介
Rapid CO2 hydrate formation was investigated with the objective of producing a negatively buoyant CO2−seawater mixture under high-pressure and low-temperature conditions, simulating direct CO2 injection at intermediate ocean depths of 1.0−1.3 km. A coflow reactor was developed to maximize CO2 hydrate production by injecting water droplets (e.g., ∼267 μm average diameter) from a capillary tube into liquid CO2. The droplets were injected in the mixing zone of the reactor where CO2 hydrate formed at the surface of the water droplets. The water-encased hydrate particles aggregated in the liquid CO2, producing a paste-like composite containing CO2 hydrate, liquid CO2, and water phases. This composite was extruded into ambient water from the coflow reactor as a coherent cylindrical mass, approximately 6 mm in diameter, which broke into pieces 5−10 cm long. Both modeling and experiments …
引用总数
20042005200620072008200920102011201220132014201520162017201820192020202120222023202456851013116595137675741053
学术搜索中的文章
S Lee, L Liang, D Riestenberg, OR West, C Tsouris… - Environmental science & technology, 2003