作者
Bo Zheng, Qiang Zhang, Dan Tong, Chuchu Chen, Chaopeng Hong, Meng Li, Guannan Geng, Yu Lei, Hong Huo, Kebin He
发表日期
2017/1/20
期刊
Atmospheric Chemistry and Physics
卷号
17
期号
2
页码范围
921-933
出版商
Copernicus GmbH
简介
Gridded emission inventories are essential inputs for chemical transport models and climate models. Spatial proxies are applied to allocate emissions from regional totals to spatially resolved grids when the exact locations of emissions are absent, with additional uncertainties arising due to the spatial mismatch between the locations of emissions and spatial proxies. In this study, we investigate the impact of spatial proxies on the accuracy of gridded emission inventories at different spatial resolutions by comparing gridded emissions developed from different spatial proxies (proxy-based inventory) with a highly spatially disaggregated bottom-up emission inventory developed from the extensive use of locations of emitting facilities (bottom-up inventory) in Hebei Province, China. We find that proxy-based inventories are generally comparable to bottom-up inventories for grid sizes larger than 0.25° because spatial errors are largely diminished at coarse resolutions. However, for gridded emissions with finer resolutions, large positive biases in urban centers and negative biases in suburban and rural regions are identified in proxy-based inventories and are then propagated into significant biases in urban-scale chemical transport modeling. Compared to bottom-up inventories, the use of proxy-based emissions exhibits similar modeling results, with biases varying from 3 to 13 % when predicting surface concentrations of different pollutants at 36 km resolution and an additional 8–73 % at 4 km resolution. The resolution dependence of uncertainties in proxy-based gridded inventories can be explained by the decoupling of emission facility locations …
引用总数
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