Generation and multi-octave shaping of mid-infrared intense single-cycle pulses

P Krogen, H Suchowski, H Liang, N Flemens… - Nature …, 2017 - nature.com
Nature Photonics, 2017nature.com
The generation of intense mid-infrared (mid-IR) optical pulses with customizable shape and
spectra spanning a multiple-octave range of vibrational frequencies is an elusive
technological capability. While some recent approaches to mid-IR supercontinuum
generation—such as filamentation, multicolour four-wave-mixing and optical rectification,,,,,,,—
have successfully generated broad spectra, no process has been identified for achieving
complex pulse shaping at the generation step. The adiabatic frequency converter, allows for …
Abstract
The generation of intense mid-infrared (mid-IR) optical pulses with customizable shape and spectra spanning a multiple-octave range of vibrational frequencies is an elusive technological capability. While some recent approaches to mid-IR supercontinuum generation—such as filamentation, multicolour four-wave-mixing and optical rectification,,,,,,,—have successfully generated broad spectra, no process has been identified for achieving complex pulse shaping at the generation step. The adiabatic frequency converter, allows for a one-to-one transfer of spectral phase through nonlinear frequency conversion over a larger-than-octave-spanning range and with an overall linear phase transfer function. Here, we show that we can convert shaped near-infrared (near-IR) pulses to shaped, energetic, multi-octave-spanning mid-IR pulses lasting only 1.2 optical cycles, and extendable to the sub-cycle regime. We expect this capability to enable a new class of precisely controlled nonlinear interactions in the mid-IR spectral range, from nonlinear vibrational spectroscopy to strong light–matter interactions and single-shot remote sensing.
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