Spin-flop transition and Zeeman effect of defect-localized bound states in the antiferromagnetic topological insulator MnBi2Te4

G Qian, M Shi, H Chen, S Zhu, J Hu, Z Huang, Y Huang… - Nano Research, 2023 - Springer
G Qian, M Shi, H Chen, S Zhu, J Hu, Z Huang, Y Huang, XH Chen, HJ Gao
Nano Research, 2023Springer
The correlation of surface impurity states with the antiferromagnetic ground states is crucial
for understanding the formation of the topological surface state in the antiferromagnetic
topological insulators MnBi2Te4. By using low-temperature scanning tunneling microscopy
and spectroscopy, we observed a localized bound state around the Mn-Bi antisite defect at
the Te-terminated surface of the antiferromagnetic topological insulator MnBi2Te4. When
applying a magnetic field perpendicular to the surface (B z) from− 1.5 to 3.0 T, the bound …
Abstract
The correlation of surface impurity states with the antiferromagnetic ground states is crucial for understanding the formation of the topological surface state in the antiferromagnetic topological insulators MnBi2Te4. By using low-temperature scanning tunneling microscopy and spectroscopy, we observed a localized bound state around the Mn-Bi antisite defect at the Te-terminated surface of the antiferromagnetic topological insulator MnBi2Te4. When applying a magnetic field perpendicular to the surface (Bz) from −1.5 to 3.0 T, the bound state shifts linearly to a lower energy with increasing Bz, which is attributed to the Zeeman effect. Remarkably, when applying a large range of Bz from −8.0 to 8.0 T, the magnetic field induced reorientation of surface magnetic moments results in an abrupt jump in the local density of states (LDOS), which is characterized by LDOS-change-ratio \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\rm{d}}\tilde \sigma /{\rm{d}}B$$\end{document} quantitatively. Interestingly, two asymmetric critical field, −2.0 and 4.0 T determined by the two peaks in \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\rm{d}}\tilde \sigma /{\rm{d}}B$$\end{document} are observed, which is consistent with simulated results according to a Mills-model, describing a surface spin flop transition (SSF). Our results provide a new flatform for studying the interplay between magnetic order and topological phases in magnetic topological materials.
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