Strong and anisotropic third-harmonic generation in monolayer and multilayer

Q Cui, RA Muniz, JE Sipe, H Zhao - Physical Review B, 2017 - APS
Q Cui, RA Muniz, JE Sipe, H Zhao
Physical Review B, 2017APS
We report observation of strong and anisotropic third-harmonic generation (THG) in
monolayer and multilayer ReS 2. The third-order nonlinear optical susceptibility of
monolayer ReS 2,| χ (3)|, is on the order of 10− 18 m 2/V 2, which is about one order of
magnitude higher than reported results for hexagonal-lattice transition metal
dichalcogenides such as MoS 2. A similar magnitude for the third-order nonlinear optical
susceptibility was also obtained for a multilayer sample. The intensity of the THG field was …
We report observation of strong and anisotropic third-harmonic generation (THG) in monolayer and multilayer . The third-order nonlinear optical susceptibility of monolayer , is on the order of , which is about one order of magnitude higher than reported results for hexagonal-lattice transition metal dichalcogenides such as . A similar magnitude for the third-order nonlinear optical susceptibility was also obtained for a multilayer sample. The intensity of the THG field was found to be dependent on the direction of the incident light polarization for both monolayer and multilayer samples. A point group symmetry analysis shows that such anisotropy is not expected from a perfect lattice and must arise from the distortions in the lattice. Our results show that THG measurements can be used to characterize lattice distortions of two-dimensional materials and that lattice distortions are important for the nonlinear optical properties of such materials.
American Physical Society
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