Ultrafast band-gap renormalization and build-up of optical gain in monolayer
Physical Review B, 2020•APS
The dynamics of band-gap renormalization and gain build-up in monolayer MoTe 2-H is
investigated by evaluating the nonequilibrium Dirac-Bloch equations with the incoherent
carrier-carrier and carrier-phonon scattering treated via quantum-Boltzmann type scattering
equations. For the case where an approximately 300-fs-long high-intensity optical pulse
generates charge-carrier densities in the gain regime, the strong Coulomb coupling leads to
a relaxation of excited carriers on a few-femtosecond timescale. The pump-pulse generation …
investigated by evaluating the nonequilibrium Dirac-Bloch equations with the incoherent
carrier-carrier and carrier-phonon scattering treated via quantum-Boltzmann type scattering
equations. For the case where an approximately 300-fs-long high-intensity optical pulse
generates charge-carrier densities in the gain regime, the strong Coulomb coupling leads to
a relaxation of excited carriers on a few-femtosecond timescale. The pump-pulse generation …
The dynamics of band-gap renormalization and gain build-up in monolayer -H is investigated by evaluating the nonequilibrium Dirac-Bloch equations with the incoherent carrier-carrier and carrier-phonon scattering treated via quantum-Boltzmann type scattering equations. For the case where an approximately 300-fs-long high-intensity optical pulse generates charge-carrier densities in the gain regime, the strong Coulomb coupling leads to a relaxation of excited carriers on a few-femtosecond timescale. The pump-pulse generation of excited carriers induces a large band-gap renormalization during the timescale of the pulse. Efficient phonon coupling leads to a subsequent carrier thermalization within a few picoseconds, which defines the timescale for the optical gain build-up energetically close to the low-density exciton resonance.
American Physical Society
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