Direct visualization of shear dependent silk fibrillogenesis

C Holland, JS Urbach, DL Blair - Soft Matter, 2012 - pubs.rsc.org
Silk's desirable properties originate from the development of a multiscale hierarchical
structure produced during spinning, but little is known regarding the origin of the micro and …

Dry-spun silk produces native-like fibroin solutions

M Boulet-Audet, C Holland, T Gheysens… - …, 2016 - ACS Publications
Silk's outstanding mechanical properties and energy efficient solidification mechanisms
provide inspiration for biomaterial self-assembly as well as offering a diverse platform of …

Mesoscale structure development reveals when a silkworm silk is spun

Q Wan, M Yang, J Hu, F Lei, Y Shuai, J Wang… - Nature …, 2021 - nature.com
Silk fibre mechanical properties are attributed to the development of a multi-scale
hierarchical structure during spinning. By careful ex vivo processing of a B. mori silkworm …

Insights into silk formation process: correlation of mechanical properties and structural evolution during artificial spinning of silk fibers

G Fang, Y Huang, Y Tang, Z Qi, J Yao… - ACS Biomaterials …, 2016 - ACS Publications
The extraordinary comprehensive mechanical properties of animal silk (especially spider
and silkworm silk) have led to extensive research on the underlying mechanisms involved …

Recombinant silk fiber properties correlate to prefibrillar self‐assembly

L Xu, N Weatherbee‐Martin, XQ Liu, JK Rainey - Small, 2019 - Wiley Online Library
Spider silks are desirable materials with mechanical properties superior to most synthetic
materials coupled with biodegradability and biocompatibility. In order to replicate natural silk …

Identification of wet-spinning and post-spin stretching methods amenable to recombinant spider aciniform silk

N Weatherbee-Martin, L Xu, A Hupe, L Kreplak… - …, 2016 - ACS Publications
Spider silks are outstanding biomaterials with mechanical properties that outperform
synthetic materials. Of the six fibrillar spider silks, aciniform (or wrapping) silk is the toughest …

Artificial spinning of natural silk threads

M Frydrych, A Greenhalgh, F Vollrath - Scientific Reports, 2019 - nature.com
Silk producing arthropods spin solid fibres from an aqueous protein feedstock apparently
relying on the complex structure of the silk protein and its controlled aggregation by shear …

Silk self-assembly mechanisms and control from thermodynamics to kinetics

Q Lu, H Zhu, C Zhang, F Zhang, B Zhang… - …, 2012 - ACS Publications
Silkworms and spiders generate fibers that exhibit high strength and extensibility. The
underlying mechanisms involved in processing silk proteins into fiber form remain …

The natural silk spinning process: A nucleation‐dependent aggregation mechanism?

G Li, P Zhou, Z Shao, X Xie, X Chen… - European Journal of …, 2001 - Wiley Online Library
The spinning mechanism of natural silk has been an open issue. In this study, both the
conformation transition from random coil to β sheet and the β sheet aggregation growth of …

Silk reconstitution disrupts fibroin self-assembly

SR Koebley, D Thorpe, P Pang… - …, 2015 - ACS Publications
Using atomic force microscopy, we present the first molecular-scale comparison of two of the
most important silk dopes, native (NSF) and reconstituted (RSF) silkworm fibroin. We found …