X-ray spectroscopy for chemical and energy sciences: the case of heterogeneous catalysis

AI Frenkel, JA van Bokhoven - Journal of synchrotron radiation, 2014 - journals.iucr.org
Heterogeneous catalysis is the enabling technology for much of the current and future
processes relevant for energy conversion and chemicals synthesis. The development of new …

Advanced X-ray absorption and emission spectroscopy: in situ catalytic studies

J Singh, C Lamberti, JA van Bokhoven - Chemical Society Reviews, 2010 - pubs.rsc.org
Knowledge of the structure of catalysts is essential to understand their behavior, which
further facilitates development of an active, selective, and stable catalyst. Determining the …

Scientific opportunities for heterogeneous catalysis research at the SuperXAS and SNBL beam lines

PM Abdala, OV Safonova, G Wiker, W van Beek… - Chimia, 2012 - chimia.ch
In this short review, we describe the complementary experimental capabilities for catalysis
research at two beam lines available to the Swiss community, SuperXAS at SLS (Swiss Light …

X-Ray Microscopy and Tomography

J Becher, T Sheppard, JD Grunwaldt - Springer Handbook of Advanced …, 2023 - Springer
Hard X-rays generated at modern synchrotron radiation sources can be exploited for a
range of X-ray imaging techniques in 2D and 3D. These methods offer unique potential for …

Reactivity of surface species in heterogeneous catalysts probed by in situ X-ray absorption techniques

S Bordiga, E Groppo, G Agostini… - Chemical …, 2013 - ACS Publications
Starting from the late seventies, the progressively increased availability of synchrotron light
sources allowed the execution of experiments requiring a high X-ray flux in a continuous …

Catalysis seen in action

M Tromp - … Transactions of the Royal Society A …, 2015 - royalsocietypublishing.org
Synchrotron radiation techniques are widely applied in materials research and
heterogeneous catalysis. In homogeneous catalysis, its use so far is rather limited despite its …

Combining synchrotron-based X-ray techniques with vibrational spectroscopies for the in situ study of heterogeneous catalysts: a view from a bridge

MA Newton, W van Beek - Chemical Society Reviews, 2010 - pubs.rsc.org
The advantages, challenges, and future possibilities for combining synchrotron-based X-ray
techniques with vibrational spectroscopies are considered in this critical review. Particular …

[PDF][PDF] A cell design for correlative hard X-ray nanoprobe and electron microscopy studies of catalysts under in situ conditions

JE Parker, M Gomez-Gonzalez… - Journal of …, 2022 - journals.iucr.org
To improve the understanding of catalysts, and ultimately the ability to design better
materials, it is crucial to study them during their catalytic active states. Using in situ or …

Hard X‐ray spectroscopic nano‐imaging of hierarchical functional materials at work

JC Andrews, BM Weckhuysen - ChemPhysChem, 2013 - Wiley Online Library
Heterogeneous catalysts often consist of an active metal (oxide) in close contact with a
support material and various promoter elements. Although macroscopic properties, such as …

Bridging the gap between the X-ray absorption spectroscopy and the computational catalysis communities in heterogeneous catalysis: a perspective on the current …

R Rana, FD Vila, AR Kulkarni, SR Bare - ACS Catalysis, 2022 - ACS Publications
X-ray absorption spectroscopy (XAS)[extended X-ray absorption fine structure (EXAFS) and
X-ray absorption near-edge structure (XANES)] is a key technique within the heterogeneous …