Adsorption and penetration of hydrogen in W: A first principles study

A Moitra, K Solanki - Computational materials science, 2011 - Elsevier
Computational materials science, 2011Elsevier
In BCC crystals, such as Tungsten (W), slippage has been observed on the (110) and (112)
planes. In this work, hydrogen diffusion paths from three different W surfaces ((100),(110)
and (112)) have been calculated using first principles density functional theory. Equilibrium
sites for H at the surfaces are identified. The energetics for H penetration from the surfaces to
the solute site in the bulk is calculated. It is found that for our low surface coverage of H (3.4×
1014H/cm2), approximately 2eV is required for an H atom to penetrate any of the W surfaces …
In BCC crystals, such as Tungsten (W), slippage has been observed on the (110) and (112) planes. In this work, hydrogen diffusion paths from three different W surfaces ((100), (110) and (112)) have been calculated using first principles density functional theory. Equilibrium sites for H at the surfaces are identified. The energetics for H penetration from the surfaces to the solute site in the bulk is calculated. It is found that for our low surface coverage of H (3.4×1014H/cm2), approximately 2eV is required for an H atom to penetrate any of the W surfaces considered in this study.
Elsevier
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