Atomic-scale strain manipulation of a charge density wave

S Gao, F Flicker, R Sankar, H Zhao… - Proceedings of the …, 2018 - National Acad Sciences
S Gao, F Flicker, R Sankar, H Zhao, Z Ren, B Rachmilowitz, S Balachandar, F Chou
Proceedings of the National Academy of Sciences, 2018National Acad Sciences
A charge density wave (CDW) is one of the fundamental instabilities of the Fermi surface
occurring in a wide range of quantum materials. In dimensions higher than one, where Fermi
surface nesting can play only a limited role, the selection of the particular wavevector and
geometry of an emerging CDW should in principle be susceptible to controllable
manipulation. In this work, we implement a simple method for straining materials compatible
with low-temperature scanning tunneling microscopy/spectroscopy (STM/S), and use it to …
A charge density wave (CDW) is one of the fundamental instabilities of the Fermi surface occurring in a wide range of quantum materials. In dimensions higher than one, where Fermi surface nesting can play only a limited role, the selection of the particular wavevector and geometry of an emerging CDW should in principle be susceptible to controllable manipulation. In this work, we implement a simple method for straining materials compatible with low-temperature scanning tunneling microscopy/spectroscopy (STM/S), and use it to strain-engineer CDWs in 2H-NbSe2. Our STM/S measurements, combined with theory, reveal how small strain-induced changes in the electronic band structure and phonon dispersion lead to dramatic changes in the CDW ordering wavevector and geometry. Our work unveils the microscopic mechanism of a CDW formation in this system, and can serve as a general tool compatible with a range of spectroscopic techniques to engineer electronic states in any material where local strain or lattice symmetry breaking plays a role.
National Acad Sciences
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