The need to optimize the performance of energy storage systems has driven the search for
new materials showing inherent properties that are favorable in enhancing energy and
power outputs. Recently, metal–organic frameworks (MOFs) have emerged as promising
materials because of their desirable features that include rich redox metal centers, rapid ion
transport, ultrahigh and tunable porosity, and large surface areas that offer maximized
electroactive sites. The electrochemical performance of MOFs depends on their architecture …