Laser-driven first-order spin reorientation and Verwey phase transitions in magnetite beyond the range of thermodynamic equilibrium

AV Kuzikova, LA Shelukhin, FM Maksimov, AI Chernov… - Physical Review B, 2023 - APS
Physical Review B, 2023APS
Ultrafast photo-induced phase transitions occurring under the impact of femtosecond laser
pulses provide versatile opportunities for switching solids between distinctly-different
crystalline, electronic, and magnetic states and thus modify their functional properties in a
significant way. In this paper, we report on the laser-induced spin reorientation and Verwey
phase transitions in a single crystalline ferrimagnetic magnetite Fe 3 O 4. Using
femtosecond optical and magneto-optical pump-probe techniques, we define the range of …
Ultrafast photo-induced phase transitions occurring under the impact of femtosecond laser pulses provide versatile opportunities for switching solids between distinctly-different crystalline, electronic, and magnetic states and thus modify their functional properties in a significant way. In this paper, we report on the laser-induced spin reorientation and Verwey phase transitions in a single crystalline ferrimagnetic magnetite . Using femtosecond optical and magneto-optical pump-probe techniques, we define the range of the initial sample temperatures and laser fluences when partial or complete photo-induced phase transitions occur from a monoclinic insulating to a cubic metallic state with concomitant switching of magnetic anisotropy from the uniaxial to the cubic one. We thus reveal a connection between these phase transitions when driven by femtosecond laser pulses. Using transient linear and quadratic magneto-optical effects, we examine magnetization dynamics launched the switching of the magnetic anisotropy axis. We unveil the presence of the domains undergoing the laser-induced phase transitions even below the established threshold fluence for the transitions, as well as when the material is initially in the cubic phase. This is the manifestation of the first order of these both laser-induced phase transitions beyond the range of thermodynamic equilibrium.
American Physical Society
以上显示的是最相近的搜索结果。 查看全部搜索结果