Spin glass behavior and colossal negative magnetoresistance of the strongly doped with phosphorus

L Van Khoi, W Dobrowolski, T Kazimierczuk, A Rodek… - Physical Review B, 2020 - APS
L Van Khoi, W Dobrowolski, T Kazimierczuk, A Rodek, P Kossacki, RR Galazka, W Zawadzki
Physical Review B, 2020APS
Magnetoresistance, ac and dc magnetization, and photoluminescence (PL) experiments
have been performed on the p-type Zn 0.99 Mn 0.01 Te and Zn 0.97 Mn 0.03 Te alloys
strongly doped with phosphorus (P). The investigated samples exhibit spin glass behavior
with ferromagnetic regions near the freezing temperature T f= 1.9 K and colossal negative
magnetoresistance (negMR) of 2.2× 10 3 times at 4.2 K for 0≤ B≤±6 T. The negMR curves
contain occurrences of hysteresis providing evidence for the memory effect. Looking for …
Magnetoresistance, ac and dc magnetization, and photoluminescence (PL) experiments have been performed on the -type and alloys strongly doped with phosphorus (P). The investigated samples exhibit spin glass behavior with ferromagnetic regions near the freezing temperature  K and colossal negative magnetoresistance (negMR) of times at 4.2 K for  T. The negMR curves contain occurrences of hysteresis providing evidence for the memory effect. Looking for possible ferromagnetic interactions responsible for the spin glass behavior at low hole densities, we observe in PL spectra that the P doping quenches internal recombination in ions. This strongly indicates a charge transfer between and ions leading to the creation of and ions. The creation of is confirmed by an observation of strong PL enhancement at excitation energies lower than the band gap and PL study at various temperatures. The resulting simultaneous existence of the mixed valence and ions can lead to double exchange mechanism of ferromagnetic interaction. Also, ions can exhibit a superexchange interaction leading to local ferromagnetic phases.
American Physical Society
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