The magnetic properties and structure of the quasi-two-dimensional antiferromagnet CoPS3
AR Wildes, V Simonet, E Ressouche… - Journal of Physics …, 2017 - iopscience.iop.org
AR Wildes, V Simonet, E Ressouche, R Ballou, GJ McIntyre
Journal of Physics: Condensed Matter, 2017•iopscience.iop.orgThe magnetic properties and magnetic structure are presented for CoPS 3, a quasi-two-
dimensional antiferromagnet on a honeycomb lattice with a Néel temperature of $ T_ {\rm
N}\sim120 $ K. The compound is shown to have XY-like anisotropy in its susceptibility, and
the anisotropy is analysed to extract crystal field parameters. For temperatures between 2 K
and 300 K, no phase transitions were observed in the field-dependent magnetization up to
10 Tesla. Single-crystal neutron diffraction shows that the magnetic propagation vector is k …
dimensional antiferromagnet on a honeycomb lattice with a Néel temperature of $ T_ {\rm
N}\sim120 $ K. The compound is shown to have XY-like anisotropy in its susceptibility, and
the anisotropy is analysed to extract crystal field parameters. For temperatures between 2 K
and 300 K, no phase transitions were observed in the field-dependent magnetization up to
10 Tesla. Single-crystal neutron diffraction shows that the magnetic propagation vector is k …
Abstract
The magnetic properties and magnetic structure are presented for CoPS 3, a quasi-two-dimensional antiferromagnet on a honeycomb lattice with a Néel temperature of K. The compound is shown to have XY-like anisotropy in its susceptibility, and the anisotropy is analysed to extract crystal field parameters. For temperatures between 2 K and 300 K, no phase transitions were observed in the field-dependent magnetization up to 10 Tesla. Single-crystal neutron diffraction shows that the magnetic propagation vector is k= with the moments mostly along the axis and with a small component along the axis, which largely verifies the previously-published magnetic structure for this compound. The magnetic Bragg peak intensity decreases with increasing temperature as a power law with exponent for .
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