From molecular to supramolecular electronics

H Chen, J Fraser Stoddart - Nature Reviews Materials, 2021 - nature.com
Using individual molecules as conducting bridges for electrons offers opportunities when
investigating quantum phenomena that are not readily accessible from experiments …

Theoretical challenges in polaritonic chemistry

J Fregoni, FJ Garcia-Vidal, J Feist - ACS photonics, 2022 - ACS Publications
Polaritonic chemistry exploits strong light–matter coupling between molecules and confined
electromagnetic field modes to enable new chemical reactivities. In systems displaying this …

Sub-nanometre resolution in single-molecule photoluminescence imaging

B Yang, G Chen, A Ghafoor, Y Zhang, Y Zhang… - Nature …, 2020 - nature.com
Ambitions to reach atomic resolution with light have been a major force in shaping nano-
optics, whereby a central challenge is achieving highly localized optical fields. A promising …

Quantum nanomagnets in on-surface metal-free porphyrin chains

Y Zhao, K Jiang, C Li, Y Liu, G Zhu, M Pizzochero… - Nature Chemistry, 2023 - nature.com
Unlike classic spins, quantum magnets are spin systems that interact via the exchange
interaction and exhibit collective quantum behaviours, such as fractional excitations …

Quantum information and algorithms for correlated quantum matter

K Head-Marsden, J Flick, CJ Ciccarino… - Chemical …, 2020 - ACS Publications
Discoveries in quantum materials, which are characterized by the strongly quantum-
mechanical nature of electrons and atoms, have revealed exotic properties that arise from …

Light–matter interaction at atomic scales

R Gutzler, M Garg, CR Ast, K Kuhnke, K Kern - Nature Reviews Physics, 2021 - nature.com
Light–matter interaction drives many systems, such as optoelectronic devices like light-
emitting diodes and solar cells, biological structures like photosystem II and potential future …

Orbital-resolved visualization of single-molecule photocurrent channels

M Imai-Imada, H Imada, K Miwa, Y Tanaka, K Kimura… - Nature, 2022 - nature.com
Given its central role in utilizing light energy, photoinduced electron transfer (PET) from an
excited molecule has been widely studied,,,,–. However, even though microscopic …

Wavelike electronic energy transfer in donor–acceptor molecular systems through quantum coherence

FF Kong, XJ Tian, Y Zhang, Y Zhang, G Chen… - Nature …, 2022 - nature.com
Quantum-coherent intermolecular energy transfer is believed to play a key role in light
harvesting in photosynthesis and photovoltaics. So far, a direct, real-space demonstration of …

Mapping Lamb, Stark, and Purcell effects at a chromophore-picocavity junction with hyper-resolved fluorescence microscopy

A Rosławska, T Neuman, B Doppagne, AG Borisov… - Physical Review X, 2022 - APS
The interactions of the excited states of a single chromophore with static and dynamic
electric fields spatially varying at the atomic scale are investigated in a joint experimental …

Strong coupling between localized surface plasmons and molecules by coupled cluster theory

J Fregoni, TS Haugland, S Pipolo, T Giovannini… - Nano Letters, 2021 - ACS Publications
Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields
within nanometric volumes. As a consequence, the molecules experience a remarkably …