Exploring the potential energy landscape of glass-forming systems: from inherent structures via metabasins to macroscopic transport
A Heuer - Journal of Physics: Condensed Matter, 2008 - iopscience.iop.org
In this review a systematic analysis of the potential energy landscape (PEL) of glass-forming
systems is presented. Starting from the thermodynamics, the route towards the dynamics is …
systems is presented. Starting from the thermodynamics, the route towards the dynamics is …
On the Adam-Gibbs-Kirkpatrick-Thirumalai-Wolynes scenario for the viscosity increase in glasses
JP Bouchaud, G Biroli - The Journal of chemical physics, 2004 - pubs.aip.org
We reformulate the interpretation of the mean-field glass transition scenario for finite
dimensional systems, proposed by Kirkpatrick, Thirumalai, and Wolynes (KTW)[Phys. Rev. A …
dimensional systems, proposed by Kirkpatrick, Thirumalai, and Wolynes (KTW)[Phys. Rev. A …
Mode-coupling theory and the glass transition in supercooled liquids
SP Das - Reviews of modern physics, 2004 - APS
Mode-coupling theory is an approach to the study of complex behavior in the supercooled
liquids which developed from the idea of a nonlinear feedback mechanism. From the …
liquids which developed from the idea of a nonlinear feedback mechanism. From the …
Density-functional theory for complex fluids
J Wu, Z Li - Annu. Rev. Phys. Chem., 2007 - annualreviews.org
Density-functional theory (DFT) and its variations provide a fruitful approach to the
computational modeling of the microscopic structures and phase behavior of soft-condensed …
computational modeling of the microscopic structures and phase behavior of soft-condensed …
Fragilities of liquids predicted from the random first order transition theory of glasses
X Xia, PG Wolynes - … of the National Academy of Sciences, 2000 - National Acad Sciences
A microscopically motivated theory of glassy dynamics based on an underlying random first
order transition is developed to explain the magnitude of free energy barriers for glassy …
order transition is developed to explain the magnitude of free energy barriers for glassy …
Density functional theory of nonuniform polyatomic systems. I. General formulation
D Chandler, JD McCoy, SJ Singer - The Journal of chemical physics, 1986 - pubs.aip.org
We extend the density functional theory of nonuniform fluids to the cases of systems
composed of polyatomic species. By the method of Legendre transforms, one demonstrates …
composed of polyatomic species. By the method of Legendre transforms, one demonstrates …
[HTML][HTML] Configurational entropy of glass-forming liquids
The configurational entropy is one of the most important thermodynamic quantities
characterizing supercooled liquids approaching the glass transition. Despite decades of …
characterizing supercooled liquids approaching the glass transition. Despite decades of …
Density-functional theory of freezing and properties of the ordered phase
Y Singh - Physics Reports, 1991 - Elsevier
We review a theory of freezing based on the density-functional approach andcompare a
variety of its versions. The application of the theory to the freezing of various simple and …
variety of its versions. The application of the theory to the freezing of various simple and …
The shapes of cooperatively rearranging regions in glass-forming liquids
The cooperative rearrangement of groups of many molecules has long been thought to
underlie the dramatic slowing of liquid dynamics on cooling towards the glassy state. For …
underlie the dramatic slowing of liquid dynamics on cooling towards the glassy state. For …
Entropic barriers, activated hopping, and the glass transition in colloidal suspensions
KS Schweizer, EJ Saltzman - The Journal of chemical physics, 2003 - pubs.aip.org
A microscopic kinetic description of single-particle transient localization and activated
transport in glassy fluids is developed which combines elements of idealized mode-coupling …
transport in glassy fluids is developed which combines elements of idealized mode-coupling …