The Optimized Catalytic Performance of Single‐Atom Catalysts by Incorporating Atomic Clusters or Nanoparticles: In‐Depth Understanding on Their Synergisms

F Mo, Q Zhou, W Xue, W Liu, S Xu… - Advanced Energy …, 2023 - Wiley Online Library
The performance optimization of single‐atom catalysts (SACs) is important but remains
challenging. Taking advantage of accompanying in situ formation of atomic clusters …

Advanced nanopesticides: advantage and action mechanisms

X Li, Y Chen, J Xu, I Lynch, Z Guo, C Xie… - Plant Physiology and …, 2023 - Elsevier
The use of various chemical substances to control pests, diseases, and weeds in the field is
a necessary part of the agricultural development process in every country. While the …

Facilely tuning the first-shell coordination microenvironment in iron single-atom for Fenton-like chemistry toward highly efficient wastewater purification

Z Wu, B Huang, X Wang, CS He, Y Liu… - Environmental …, 2023 - ACS Publications
Precisely identifying the atomic structures in single-atom sites and establishing authentic
structure–activity relationships for single-atom catalyst (SAC) coordination are significant …

Fenton-like activity and pathway modulation via single-atom sites and pollutants comediates the electron transfer process

J Guo, Y Wang, Y Shang, K Yin, Q Li… - Proceedings of the …, 2024 - National Acad Sciences
The studies on the origin of versatile oxidation pathways toward targeted pollutants in the
single-atom catalysts (SACs)/peroxymonosulfate (PMS) systems were always associated …

Regulating the Local Electronic Structure of Copper Single Atoms with Unsaturated B,O-Coordination for Selective 1O2 Generation

P Yang, Z Cao, Y Long, D Liu, W Huang, S Zhan… - ACS …, 2023 - ACS Publications
Generating singlet oxygen (1O2) on single atom catalysts (SACs) in peroxymonosulfate
(PMS)-based Fenton-like reactions exhibits great potential for selective degradation of …

In situ ligand-modulated activation of inert Ce (III/IV) into ozonation catalyst for efficient water treatment

J Zhang, C Shan, W Zhang… - Proceedings of the …, 2023 - National Acad Sciences
As a classic strategy to maximize catalytic activity, modulation of the electronic structure of
central metal using organic ligands encounters great challenge in radical reactions …

Efficient Removal of Antibiotic Resistance Genes through 4f‐2p‐3d Gradient Orbital Coupling Mediated Fenton‐Like Redox Processes

F Li, P Wang, T Zhang, M Li, S Yue… - Angewandte …, 2023 - Wiley Online Library
Peroxymonosulfate (PMS) mediated radical and nonradical active substances can
synergistically achieve the efficient elimination of antibiotic resistance genes (ARGs) …

Single cobalt atoms anchored on Ti3C2Tx with dual reaction sites for efficient adsorption–degradation of antibiotic resistance genes

M Li, P Wang, K Zhang, H Zhang… - Proceedings of the …, 2023 - National Acad Sciences
The assimilation of antibiotic resistance genes (ARGs) by pathogenic bacteria poses a
severe threat to public health. Here, we reported a dual-reaction-site–modified …

[HTML][HTML] Tailoring d-band center of high-valent metal-oxo species for pollutant removal via complete polymerization

HZ Liu, XX Shu, M Huang, BB Wu, JJ Chen… - Nature …, 2024 - nature.com
Polymerization-driven removal of pollutants in advanced oxidation processes (AOPs) offers
a sustainable way for the simultaneous achievement of contamination abatement and …

Selective hydroxyl generation for efficient pollutant degradation by electronic structure modulation at Fe sites

H Zhan, R Zhou, P Wang… - Proceedings of the …, 2023 - National Acad Sciences
Hydrogen peroxide (H2O2) is an important green oxidant in the field of sewage treatment,
and how to improve its activation efficiency and generate free radicals with stronger …