Visualizing vibrational normal modes of a single molecule with atomically confined light

J Lee, KT Crampton, N Tallarida, VA Apkarian - Nature, 2019 - nature.com
The internal vibrations of molecules drive the structural transformations that underpin
chemistry and cellular function. While vibrational frequencies are measured by …

Chemical mapping of a single molecule by plasmon-enhanced Raman scattering

R Zhang, Y Zhang, ZC Dong, S Jiang, C Zhang… - Nature, 2013 - nature.com
Visualizing individual molecules with chemical recognition is a longstanding target in
catalysis, molecular nanotechnology and biotechnology. Molecular vibrations provide a …

Super-multiplex vibrational imaging

L Wei, Z Chen, L Shi, R Long, AV Anzalone, L Zhang… - Nature, 2017 - nature.com
The ability to visualize directly a large number of distinct molecular species inside cells is
increasingly essential for understanding complex systems and processes. Even though …

Selectivity in vibrationally mediated single-molecule chemistry

JI Pascual, N Lorente, Z Song, H Conrad, HP Rust - Nature, 2003 - nature.com
The selective excitation of molecular vibrations provides a means to directly influence the
speed and outcome of chemical reactions. Such mode-selective chemistry has traditionally …

Trapping an atom with single photons

PWH Pinkse, T Fischer, P Maunz, G Rempe - Nature, 2000 - nature.com
The creation of a photon–atom bound state was first envisaged for the case of an atom in a
long-lived excited state inside a high-quality microwave cavity,. In practice, however, light …

Tracking the ultrafast motion of a single molecule by femtosecond orbital imaging

TL Cocker, D Peller, P Yu, J Repp, R Huber - Nature, 2016 - nature.com
Watching a single molecule move on its intrinsic timescale has been one of the central goals
of modern nanoscience, and calls for measurements that combine ultrafast temporal …

Visualizing and controlling vibrational wave packets of single molecules

D Brinks, FD Stefani, F Kulzer, R Hildner, TH Taminiau… - Nature, 2010 - nature.com
The active steering of the pathways taken by chemical reactions and the optimization of
energy conversion processes,, provide striking examples of the coherent control of quantum …

A prototype storage ring for neutral molecules

FMH Crompvoets, HL Bethlem, RT Jongma, G Meijer - Nature, 2001 - nature.com
The ability to cool and manipulate atoms with light has yielded atom interferometry, precision
spectroscopy, Bose–Einstein condensates and atom lasers. The extension of controlled …

Sub-cycle atomic-scale forces coherently control a single-molecule switch

D Peller, LZ Kastner, T Buchner, C Roelcke, F Albrecht… - Nature, 2020 - nature.com
Scanning probe techniques can leverage atomically precise forces to sculpt matter at
surfaces, atom by atom. These forces have been applied quasi-statically to create surface …

Amplitude spectroscopy of a solid-state artificial atom

DM Berns, MS Rudner, SO Valenzuela, KK Berggren… - Nature, 2008 - nature.com
The energy-level structure of a quantum system, which has a fundamental role in its
behaviour, can be observed as discrete lines and features in absorption and emission …