Graphene at liquid copper catalysts: atomic‐scale agreement of experimental and first‐principles adsorption height

H Gao, V Belova, F La Porta, JS Cingolani… - Advanced …, 2022 - Wiley Online Library
Liquid metal catalysts have recently attracted attention for synthesizing high‐quality 2D
materials facilitated via the catalysts' perfectly smooth surface. However, the microscopic …

In situ characterisation of graphene growth on liquid copper-gallium alloys: Paving the path for cost-effective synthesis

V Rein, F Letellier, M Jankowski, M de Voogd… - Applied Surface …, 2024 - Elsevier
Liquid metal catalysts (LMCats), primarily molten copper, have demonstrated their efficiency
in the chemical vapour deposition (CVD) approach for synthesising highquality, large-area …

Interface between graphene and liquid Cu from molecular dynamics simulations

JS Cingolani, M Deimel, S Köcher… - The Journal of …, 2020 - pubs.aip.org
Controllable synthesis of defect-free graphene is crucial for applications since the properties
of graphene are highly sensitive to any deviations from the crystalline lattice. We focus here …

Discovery of Graphene Growth Alloy Catalysts Using High-Throughput Machine Learning

X Li, JQ Shi, AJ Page - Nano Letters, 2023 - ACS Publications
Despite today's commercial-scale graphene production using chemical vapor deposition
(CVD), the growth of high-quality single-layer graphene with controlled morphology and …

Ab initio thermodynamics of hydrocarbons relevant to graphene growth at solid and liquid Cu surfaces

M Andersen, JS Cingolani, K Reuter - The Journal of Physical …, 2019 - ACS Publications
Using ab initio thermodynamics, the stability of a wide range of hydrocarbon adsorbates
under various chemical vapor deposition (CVD) conditions (temperature, methane and …

Development of a reactor for the in situ monitoring of 2D materials growth on liquid metal catalysts, using synchrotron x-ray scattering, Raman spectroscopy, and …

M Saedi, JM De Voogd, A Sjardin, A Manikas… - Review of Scientific …, 2020 - pubs.aip.org
Liquid metal catalysts (LMCats)(eg, molten copper) can provide a new mass-production
method for two-dimensional materials (2DMs)(eg, graphene) with significantly higher quality …

Graphene nucleation on a surface-molten copper catalyst: quantum chemical molecular dynamics simulations

HB Li, AJ Page, C Hettich, B Aradi, C Köhler… - Chemical …, 2014 - pubs.rsc.org
Chemical vapor deposition (CVD) growth of graphene on Cu (111) has been modeled with
quantum chemical molecular dynamics (QM/MD) simulations. These simulations …

Real-time multiscale monitoring and tailoring of graphene growth on liquid copper

M Jankowski, M Saedi, F La Porta, AC Manikas… - Acs Nano, 2021 - ACS Publications
The synthesis of large, defect-free two-dimensional materials (2DMs) such as graphene is a
major challenge toward industrial applications. Chemical vapor deposition (CVD) on liquid …

Controllable fabrication of graphene and related two-dimensional materials on liquid metals via chemical vapor deposition

M Zeng, L Fu - Accounts of chemical research, 2018 - ACS Publications
Conspectus Due to the confinement of the charge, spin, and heat transport in the plane,
graphene and related two-dimensional (2D) materials have been demonstrated to own …

Comparing graphene growth on Cu (111) versus oxidized Cu (111)

S Gottardi, K Müller, L Bignardi, JC Moreno-López… - Nano …, 2015 - ACS Publications
The epitaxial growth of graphene on catalytically active metallic surfaces via chemical vapor
deposition (CVD) is known to be one of the most reliable routes toward high-quality large …