Electrochemistry and capacitive charging of porous electrodes in asymmetric multicomponent electrolytes
We present porous electrode theory for the general situation of electrolytes containing
mixtures of mobile ions of arbitrary valencies and diffusion coefficients (mobilities). We focus …
mixtures of mobile ions of arbitrary valencies and diffusion coefficients (mobilities). We focus …
Time-dependent ion selectivity in capacitive charging of porous electrodes
In a combined experimental and theoretical study, we show that capacitive charging of
porous electrodes in multicomponent electrolytes may lead to the phenomenon of time …
porous electrodes in multicomponent electrolytes may lead to the phenomenon of time …
Diffuse charge and Faradaic reactions in porous electrodes
Porous electrodes instead of flat electrodes are widely used in electrochemical systems to
boost storage capacities for ions and electrons, to improve the transport of mass and charge …
boost storage capacities for ions and electrons, to improve the transport of mass and charge …
Nonlinear dynamics of capacitive charging and desalination by porous electrodes
PM Biesheuvel, MZ Bazant - Physical Review E—Statistical, Nonlinear, and …, 2010 - APS
The rapid and efficient exchange of ions between porous electrodes and aqueous solutions
is important in many applications, such as electrical energy storage by supercapacitors …
is important in many applications, such as electrical energy storage by supercapacitors …
Effective ion diffusion in charged nanoporous materials
X Zhang, DM Tartakovsky - Journal of The Electrochemical …, 2017 - iopscience.iop.org
Multiscale models of ion transport in porous media relate microscopic material properties
(eg, pore size distribution and pore connectivity) to their macroscopic counterparts (eg …
(eg, pore size distribution and pore connectivity) to their macroscopic counterparts (eg …
Analysis of non-uniform charge/discharge and rate effects in porous carbon capacitors containing sub-optimal electrolyte concentrations
WG Pell, BE Conway, N Marincic - Journal of electroanalytical chemistry, 2000 - Elsevier
The effects of internal electrolyte resistance on the acceptance and delivery of charge by a
series of 3 V, non-aqueous, double-layer capacitors have been investigated by cyclic …
series of 3 V, non-aqueous, double-layer capacitors have been investigated by cyclic …
Charge efficiency: a functional tool to probe the double-layer structure inside of porous electrodes and application in the modeling of capacitive deionization
R Zhao, PM Biesheuvel, H Miedema… - The Journal of …, 2010 - ACS Publications
Porous electrodes are important in many physical− chemical processes including capacitive
deionization (CDI), a desalination technology where ions are adsorbed from solution into the …
deionization (CDI), a desalination technology where ions are adsorbed from solution into the …
Multiphase porous electrode theory
Porous electrode theory, pioneered by John Newman and collaborators, provides a
macroscopic description of battery cycling behavior, rooted in microscopic physical models …
macroscopic description of battery cycling behavior, rooted in microscopic physical models …
Equilibria model for pH variations and ion adsorption in capacitive deionization electrodes
Ion adsorption and equilibrium between electrolyte and microstructure of porous electrodes
are at the heart of capacitive deionization (CDI) research. Surface functional groups are …
are at the heart of capacitive deionization (CDI) research. Surface functional groups are …
Ions transport and adsorption mechanisms in porous electrodes during capacitive-mixing double layer expansion (CDLE)
A model of the electro-diffusion of ions in porous electrodes is applied to analyze the
dynamics of capacitive-mixing extraction of energy from salinity gradients with carbon …
dynamics of capacitive-mixing extraction of energy from salinity gradients with carbon …
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