Bioinspired multiscale micro-/nanofiber network design enabling extremely compressible, fatigue-resistant, and rapidly shape-recoverable cryogels

L Qi, S Wang, L Chen, L Yu, X Guo, M Chen… - ACS …, 2023 - ACS Publications
Cryogels with extreme mechanical properties such as ultrahigh compressibility, fatigue
resistance, and rapid recovery are attractive in biomedical, environmental remediation, and …

Fabrication of anisotropic silk fibroin-cellulose nanocrystals cryogels with tunable mechanical properties, rapid swelling, and structural recoverability via a directional …

R Dai, L Meng, Q Fu, S Hao, J Yang - ACS Sustainable Chemistry …, 2021 - ACS Publications
A hierarchically anisotropic structure is widely found in natural materials, such as tendons
and wood for performing specific functions. However, fabrication of anisotropic materials …

Strong and tough fibrous hydrogels reinforced by multiscale hierarchical structures with multimechanisms

X Guo, X Dong, G Zou, H Gao, W Zhai - Science Advances, 2023 - science.org
Tough natural materials such as nacre, bone, and silk exhibit multiscale hierarchical
structures where distinct toughening mechanisms occur at each level of the hierarchy …

Robust multiscale-oriented thermoresponsive fibrous hydrogels with rapid self-recovery and ultrafast response underwater

Q Mu, Q Zhang, W Yu, M Su, Z Cai, K Cui… - … applied materials & …, 2020 - ACS Publications
Hydrogels with ultrafast response to environmental stimuli, possessing robust structural
integrity and rapid self-recovery, have been considered as promising platforms for numerous …

[HTML][HTML] Aqueous spinning of robust, self-healable, and crack-resistant hydrogel microfibers enabled by hydrogen bond nanoconfinement

Y Shi, B Wu, S Sun, P Wu - Nature Communications, 2023 - nature.com
Robust damage-tolerant hydrogel fibers with high strength, crack resistance, and self-
healing properties are indispensable for their long-term uses in soft machines and robots as …

Tunable biomimetic hydrogels from silk fibroin and nanocellulose

P Dorishetty, R Balu, SS Athukoralalage… - ACS Sustainable …, 2020 - ACS Publications
Biomimetic hydrogels offer a new platform for hierarchical structure-controlled, tough,
biocompatible, mechanically tunable, and printable gels for regenerative medicine. Herein …

[HTML][HTML] Bioinspired structural hydrogels with highly ordered hierarchical orientations by flow-induced alignment of nanofibrils

S Zhu, S Wang, Y Huang, Q Tang, T Fu, R Su… - Nature …, 2024 - nature.com
Natural structural materials often possess unique combinations of strength and toughness
resulting from their complex hierarchical assembly across multiple length scales. However …

A universal strategy for preparing tough and smart glassy hydrogels

X Lin, X Wang, H Cui, G Ouyang, H Guo - Chemical Engineering Journal, 2023 - Elsevier
With a large amount of water as plasticizer, most current hydrogels stay in rubbery states
with low rigidity. Inspired by the robust thermoplastics, herein we propose a facile, effective …

Eco-friendly carboxymethyl cellulose nanofiber hydrogels prepared via freeze cross-linking and their applications

Y Sekine, T Nankawa, S Yunoki, T Sugita… - ACS Applied Polymer …, 2020 - ACS Publications
We developed a cross-linking method using freeze concentration and used it to synthesize a
carboxymethyl cellulose nanofiber (CMCF) hydrogel with high water content (> 94%), high …

Macroporous silk nanofiber cryogels with tunable properties

X Zhang, Y Hang, Z Ding, L Xiao, W Cheng… - …, 2022 - ACS Publications
Cryogels are widely used in tissue regeneration due to their porous structures and friendly
hydrogel performance. Silk-based cryogels were developed but failed to exhibit desirable …