Intermolecular forces at ice and water interfaces: Premelting, surface freezing, and regelation

J Luengo-Márquez, F Izquierdo-Ruiz… - The Journal of …, 2022 - pubs.aip.org
Using Lifshitz theory, we assess the role of van der Waals forces at interfaces of ice and
water. The results are combined with measured structural forces from computer simulations …

Impurity effects in the premelting of ice

JS Wettlaufer - Physical Review Letters, 1999 - APS
The effect of impurities on the surface and interfacial melting of ice is investigated in the
context of the Derjaguin-Landau-Verwey-Overbeek theory by calculating van der Waals and …

Rounded layering transitions on the surface of ice

P Llombart, EG Noya, DN Sibley, AJ Archer… - Physical Review Letters, 2020 - APS
Understanding the wetting properties of premelting films requires knowledge of the film's
equation of state, which is not usually available. Here we calculate the disjoining pressure …

Why is it so difficult to identify the onset of ice premelting?

Y Qiu, V Molinero - The journal of physical chemistry letters, 2018 - ACS Publications
Premelting of ice at temperatures below 0° C is of fundamental importance for environmental
processes. Various experimental techniques have been used to investigate the temperature …

Dispersion-force effects in interfacial premelting of ice

LA Wilen, JS Wettlaufer, M Elbaum, M Schick - Physical Review B, 1995 - APS
We calculate the van der Waals contribution to the surface free energy of ice-water-substrate
systems as a model for interfacial melting. The result for each substrate is the excess surface …

Premelting of ice adsorbed on a rock surface

V Esteso, S Carretero-Palacios… - Physical Chemistry …, 2020 - pubs.rsc.org
Considering ice-premelting on a quartz rock surface (ie silica) we calculate the Lifshitz
excess pressures in a four layer system with rock–ice–water–air. Our calculations give …

Premelting dynamics: Geometry and interactions

JS Wettlaufer, MG Worster, LA Wilen - The Journal of Physical …, 1997 - ACS Publications
Recent advances in understanding the evolution of interfacially melted water films are
discussed from several perspectives. The essential mechanism is the motion of thin films …

Thermodynamic origin of surface melting on ice crystals

K Murata, H Asakawa, K Nagashima… - Proceedings of the …, 2016 - National Acad Sciences
Since the pioneering prediction of surface melting by Michael Faraday, it has been widely
accepted that thin water layers, called quasi-liquid layers (QLLs), homogeneously and …

Closer look at the surface of ice

DT Limmer - Proceedings of the National Academy of …, 2016 - National Acad Sciences
When hydrogen bonds are broken at an interface, water molecules are forced to adopt
configurations that are not as energetically favorable as those deep within the bulk of the …

The surface of ice under equilibrium and nonequilibrium conditions

Y Nagata, T Hama, EHG Backus… - Accounts of chemical …, 2019 - ACS Publications
Conspectus The ice premelt, often called the quasi-liquid layer (QLL), is key for the
lubrication of ice, gas uptake by ice, and growth of aerosols. Despite its apparent …