Electrons dynamics control by shaping femtosecond laser pulses in micro/nanofabrication: modeling, method, measurement and application

L Jiang, AD Wang, B Li, TH Cui, YF Lu - Light: Science & Applications, 2018 - nature.com
During femtosecond laser fabrication, photons are mainly absorbed by electrons, and the
subsequent energy transfer from electrons to ions is of picosecond order. Hence, lattice …

The ultrafast X-ray spectroscopic revolution in chemical dynamics

PM Kraus, M Zürch, SK Cushing, DM Neumark… - Nature Reviews …, 2018 - nature.com
The past two decades have seen rapid developments in short-pulse X-ray sources, which
have enabled the study of nuclear and electronic dynamics by ultrafast X-ray spectroscopies …

Measurement and laser control of attosecond charge migration in ionized iodoacetylene

PM Kraus, B Mignolet, D Baykusheva, A Rupenyan… - Science, 2015 - science.org
The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a
broad range of chemical and biophysical processes. We advanced high-harmonic …

[HTML][HTML] Charge migration and charge transfer in molecular systems

HJ Wörner, CA Arrell, N Banerji, A Cannizzo… - Structural …, 2017 - pubs.aip.org
The transfer of charge at the molecular level plays a fundamental role in many areas of
chemistry, physics, biology and materials science. Today, more than 60 years after the …

Electric-/magnetic-field-assisted photocatalysis: Mechanisms and design strategies

Z Wang, Y Li, C Wu, SCE Tsang - Joule, 2022 - cell.com
Photocatalysis as a promising approach for solar energy conversion has attracted enormous
attention in recent decades with various chemical reactions involved. Many strategies and …

Attosecond imaging of molecules using high harmonic spectroscopy

P Peng, C Marceau, DM Villeneuve - Nature Reviews Physics, 2019 - nature.com
The availability of attosecond-duration extreme ultraviolet or soft X-ray light sources has
opened up new fields of research in atomic and molecular physics. These pulses can be as …

How oriented external electric fields modulate reactivity

S Yu, P Vermeeren, TA Hamlin… - … –A European Journal, 2021 - Wiley Online Library
A judiciously oriented external electric field (OEEF) can catalyze a wide range of reactions
and can even induce endo/exo stereoselectivity of cycloaddition reactions. The Diels–Alder …

Near-forward rescattering photoelectron holography in strong-field ionization: extraction of the phase of the scattering amplitude

Y Zhou, OI Tolstikhin, T Morishita - Physical Review Letters, 2016 - APS
We revisit the concept of near-forward rescattering strong-field photoelectron holography
introduced by Y. Huismans et al.[Science 331, 61 (2011)]. The recently developed adiabatic …

Real-time probing of chirality during a chemical reaction

D Baykusheva, D Zindel, V Svoboda… - Proceedings of the …, 2019 - National Acad Sciences
Chiral molecules interact and react differently with other chiral objects, depending on their
handedness. Therefore, it is essential to understand and ultimately control the evolution of …

Perspectives of attosecond spectroscopy for the understanding of fundamental electron correlations

PM Kraus, HJ Wörner - Angewandte Chemie International …, 2018 - Wiley Online Library
The description of the electronic structure of molecules in terms of molecular orbitals is a
highly successful concept in chemistry. However, it commonly fails if the electrons in a …