Ultrafast electron diffraction: Visualizing dynamic states of matter

D Filippetto, P Musumeci, RK Li, BJ Siwick… - Reviews of Modern …, 2022 - APS
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …

Ultrafast dynamics of electrons and phonons: from the two-temperature model to the time-dependent Boltzmann equation

F Caruso, D Novko - Advances in Physics: X, 2022 - Taylor & Francis
The advent of pump-probe spectroscopy techniques paved the way to the exploration of
ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption …

Electron-phonon coupling and energy flow in a simple metal beyond the two-temperature approximation

L Waldecker, R Bertoni, R Ernstorfer, J Vorberger - Physical Review X, 2016 - APS
The electron-phonon coupling and the corresponding energy exchange are investigated
experimentally and by ab initio theory in nonequilibrium states of the free-electron metal …

Light-induced picosecond rotational disordering of the inorganic sublattice in hybrid perovskites

X Wu, LZ Tan, X Shen, T Hu, K Miyata, MT Trinh… - Science …, 2017 - science.org
Femtosecond resolution electron scattering techniques are applied to resolve the first atomic-
scale steps following absorption of a photon in the prototypical hybrid perovskite …

Direct View of Phonon Dynamics in Atomically Thin MoS2

TL Britt, Q Li, LP René de Cotret, N Olsen, M Otto… - Nano Letters, 2022 - ACS Publications
Transition-metal dichalcogenide monolayers and heterostructures are highly tunable
material systems that provide excellent models for physical phenomena at the two …

Direct observation of strong momentum-dependent electron-phonon coupling in a metal

M Mo, A Tamm, E Metsanurk, Z Chen, L Wang… - Science …, 2024 - science.org
Phonon scattering in metals is one of the most fundamental processes in materials science.
However, understanding such processes has remained challenging and requires detailed …

Theory of out-of-equilibrium ultrafast relaxation dynamics in metals

P Maldonado, K Carva, M Flammer, PM Oppeneer - Physical Review B, 2017 - APS
Ultrafast laser excitation of a metal causes correlated, highly nonequilibrium dynamics of
electronic and ionic degrees of freedom, which are, however, only poorly captured by the …

Ultrafast lattice disordering can be accelerated by electronic collisional forces

GA de la Peña Muñoz, AA Correa, S Yang, O Delaire… - Nature Physics, 2023 - nature.com
In the prevalent picture of ultrafast structural phase transitions, atomic motion occurs in a
slowly varying potential energy surface adiabatically determined by fast electrons. However …

Momentum-Resolved View of Electron-Phonon Coupling in Multilayer

L Waldecker, R Bertoni, H Hübener, T Brumme… - Physical Review Letters, 2017 - APS
We investigate the interactions of photoexcited carriers with lattice vibrations in thin films of
the layered transition metal dichalcogenide (TMDC) WSe 2. Employing femtosecond …

A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes

WH Li, CJR Duncan, MB Andorf, AC Bartnik… - Structural …, 2022 - pubs.aip.org
We report the design and performance of a time-resolved electron diffraction apparatus
capable of producing intense bunches with simultaneously single digit micrometer probe …