Single-molecule optics

F Kulzer, M Orrit - Annu. Rev. Phys. Chem., 2004 - annualreviews.org
▪ Abstract We review recent developments in single-molecule spectroscopy and microscopy.
New optical methods provide access to the absorption, emission, or excitation spectra of …

[图书][B] Generalized gaussian structures: Models for polymer systems with complextopologies

AA Gurtovenko, A Blumen - 2005 - Springer
A fundamental and long-standing problem in polymer physics is to deduce the relationship
between the topology of a polymer and its dynamics. Generalized Gaussian structures …

Weak ergodicity breaking of receptor motion in living cells stemming from random diffusivity

C Manzo, JA Torreno-Pina, P Massignan… - Physical Review X, 2015 - APS
Molecular transport in living systems regulates numerous processes underlying biological
function. Although many cellular components exhibit anomalous diffusion, only recently has …

Digital photoswitching of fluorescence based on the photochromism of diarylethene derivatives at a single-molecule level

T Fukaminato, T Sasaki, T Kawai… - Journal of the American …, 2004 - ACS Publications
Photochromic reactions of diarylethene derivatives were detected at a single-molecule level
by using a fluorescence technique. Fluorescent photoswitching molecules in which …

The energy gap law at work: Emission yield and rate fluctuations of single NIR emitters

C Erker, T Basché - Journal of the American Chemical Society, 2022 - ACS Publications
Internal conversion (IC) often is the dominating relaxation pathway in NIR emitters, lowering
their fluorescence quantum yield. Here, we investigate dibenzoterrylene (DBT) by bulk and …

Photochromism of diarylethene single molecules in polymer matrices

T Fukaminato, T Umemoto, Y Iwata… - Journal of the …, 2007 - ACS Publications
Robust fluorescent photoswitching molecules, having perylene bisimide as the fluorescent
unit and diarylethene as the switching unit, were prepared, and their photochromic reactions …

Ultrafast dynamics of single molecules

D Brinks, R Hildner, EMHP Van Dijk… - Chemical Society …, 2014 - pubs.rsc.org
The detection of individual molecules has found widespread application in molecular
biology, photochemistry, polymer chemistry, quantum optics and super-resolution …

Micro-refractometry and local-field mapping with single molecules

AV Naumov, AA Gorshelev, MG Gladush… - Nano Letters, 2018 - ACS Publications
The refractive index n is one of the most important materials parameters of solids and, in
recent years, has become the subject of significant interdisciplinary interest, especially in …

Statistical evaluation of single nano‐object fluorescence

M Lippitz, F Kulzer, M Orrit - ChemPhysChem, 2005 - Wiley Online Library
Single nano‐objects display strong fluctuations of their fluorescence signals. These random
and irreproducible variations must be subject to statistical analysis to provide microscopic …

Visualizing spatial and temporal heterogeneity of single molecule rotational diffusion in a glassy polymer by defocused wide-field imaging

H Uji-i, SM Melnikov, A Deres, G Bergamini… - Polymer, 2006 - Elsevier
Defocused wide-field fluorescence microscopy was used to follow the 3D molecular
rotational diffusion of a fluorescent probe molecule in a polymer thin film. The technique …