Time-resolved experiments on gas-phase atoms and molecules with XUV and X-ray free-electron lasers

D Rolles - Advances in Physics: X, 2023 - Taylor & Francis
Over the last 20 years, XUV and X-ray free-electron lasers have enabled a wide variety of
time-resolved experiments that have dramatically advanced our understanding of ultrafast …

Atomic, molecular and optical physics applications of longitudinally coherent and narrow bandwidth Free-Electron Lasers

C Callegari, AN Grum-Grzhimailo, KL Ishikawa… - Physics Reports, 2021 - Elsevier
Abstract Short wavelength Free-Electron Lasers (FELs) are among the newest light sources
available to scientists to probe a wide range of phenomena, with chemical, physical and …

Attosecond coherent control of electronic wave packets in two-colour photoionization using a novel timing tool for seeded free-electron laser

PK Maroju, M Di Fraia, O Plekan, M Bonanomi… - Nature …, 2023 - nature.com
In ultrafast spectroscopy, the temporal resolution of time-resolved experiments depends on
the duration of the pump and probe pulses, and on the control and characterization of their …

Atomic partial wave meter by attosecond coincidence metrology

W Jiang, GSJ Armstrong, J Tong, Y Xu, Z Zuo… - Nature …, 2022 - nature.com
Attosecond chronoscopy is central to the understanding of ultrafast electron dynamics in
matter from gas to the condensed phase with attosecond temporal resolution. It has …

Influence of shape resonances on the angular dependence of molecular photoionization delays

F Holzmeier, J Joseph, JC Houver, M Lebech… - Nature …, 2021 - nature.com
Characterizing time delays in molecular photoionization as a function of the ejected electron
emission direction relative to the orientation of the molecule and the light polarization axis …

Femtosecond polarization shaping of free-electron laser pulses

G Perosa, J Wätzel, D Garzella, E Allaria… - Physical Review Letters, 2023 - APS
We demonstrate the generation of extreme-ultraviolet (XUV) free-electron laser (FEL) pulses
with time-dependent polarization. To achieve polarization modulation on a femtosecond …

Manipulating Parallel and Perpendicular Multiphoton Transitions in Molecules

S Pan, Z Zhang, L Xu, W Zhang, P Lu, Q Ji, K Lin… - Physical Review Letters, 2023 - APS
We demonstrate that dissociative ionization of H 2 can be fully manipulated in an angle-time-
resolved fashion, employing a polarization-skewed (PS) laser pulse in which the …

Spheroidal-wave analysis of time delay in molecular reconstruction of attosecond beating by interference of two-photon transitions around a Cooper-like minimum

Q Ke, Y Zhou, Y Liao, M Li, K Liu, P Lu - Physical Review A, 2023 - APS
By numerically solving the three-dimensional time-dependent Schrödinger equation, we
have studied the energy-and angle-resolved time delay in H 2+ photoionization using the …

Control of ion-photoelectron entanglement and coherence via Rabi oscillations

KL Ishikawa, KC Prince, K Ueda - The Journal of Physical …, 2023 - ACS Publications
We report a theoretical investigation of photoionization by a pair of coherent, ultrashort,
fundamental and second-harmonic extreme-ultraviolet pulses, where the photon energies …

Unveiling Rabi dynamics through angle-resolved photoelectron momentum distributions using an pulse pair

YJ Mao, HB Yao, M He, ZH Zhang, Y Li, F He - Physical Review A, 2023 - APS
We present an interferometric method for studying the Rabi dynamics in atoms by employing
an ω-2 ω extreme ultraviolet pulse pair generated from the seeded free-electron laser. By …