Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

EW Lees, BAW Mowbray, FGL Parlane… - Nature Reviews …, 2022 - nature.com
The CO2 reduction reaction (CO2RR) is a potential means of using renewable electricity to
synthesize commodity chemicals and fuels. The CO2RR can be performed at industrially …

Conversion of CO2 to multicarbon products in strong acid by controlling the catalyst microenvironment

Y Zhao, L Hao, A Ozden, S Liu, RK Miao, P Ou… - Nature …, 2023 - nature.com
Electrosynthesis of multicarbon products from the reduction of CO2 in acidic electrolytes is a
promising approach to overcoming CO2 reactant loss in alkaline and neutral electrolytes; …

Identification of Cu(100)/Cu(111) Interfaces as Superior Active Sites for CO Dimerization During CO2 Electroreduction

ZZ Wu, XL Zhang, ZZ Niu, FY Gao… - Journal of the …, 2021 - ACS Publications
The electrosynthesis of valuable multicarbon chemicals using carbon dioxide (CO2) as a
feedstock has substantially progressed recently but still faces considerable challenges. A …

Highly selective and productive reduction of carbon dioxide to multicarbon products via in situ CO management using segmented tandem electrodes

T Zhang, JC Bui, Z Li, AT Bell, AZ Weber, J Wu - Nature Catalysis, 2022 - nature.com
Electrochemical CO2 reduction provides a promising route to the sustainable generation of
valuable chemicals and fuels. Tandem catalysts enable sequential CO2-to-CO and CO-to …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

[HTML][HTML] Enhancing carbon dioxide gas-diffusion electrolysis by creating a hydrophobic catalyst microenvironment

Z Xing, L Hu, DS Ripatti, X Hu, X Feng - Nature communications, 2021 - nature.com
Electroreduction of carbon dioxide (CO2) over copper-based catalysts provides an attractive
approach for sustainable fuel production. While efforts are focused on developing catalytic …

Interfacial Electrolyte Effects on Electrocatalytic CO2 Reduction

B Deng, M Huang, X Zhao, S Mou, F Dong - ACS Catalysis, 2021 - ACS Publications
Electrocatalytic CO2 reduction (CO2RR), powered by renewable energy, has great potential
in decreasing the concentration of CO2 in the atmosphere, as well as producing high value …

[HTML][HTML] Tunable CO2 electroreduction to ethanol and ethylene with controllable interfacial wettability

Y Lin, T Wang, L Zhang, G Zhang, L Li, Q Chang… - Nature …, 2023 - nature.com
The mechanism of how interfacial wettability impacts the CO2 electroreduction pathways to
ethylene and ethanol remains unclear. This paper describes the design and realization of …

Strategies to suppress hydrogen evolution for highly selective electrocatalytic nitrogen reduction: challenges and perspectives

Y Ren, C Yu, X Tan, H Huang, Q Wei… - Energy & Environmental …, 2021 - pubs.rsc.org
Ammonia, as a significant chemical for fertilizer production and also a promising energy
carrier, is mainly produced through the traditional energy-intensive Haber–Bosch process …