Iron photoredox catalysis–past, present, and future

LHM de Groot, A Ilic, J Schwarz… - Journal of the American …, 2023 - ACS Publications
Photoredox catalysis of organic reactions driven by iron has attracted substantial attention
throughout recent years, due to potential environmental and economic benefits. In this …

The great strides of iron photosensitizers for contemporary organic photoredox catalysis: On our way to the holy grail?

F Glaser, A Aydogan, B Elias… - Coordination Chemistry …, 2024 - Elsevier
The scarcity of 2 nd and 3 rd row transition metals such as ruthenium, iridium, rhodium and
osmium, coupled with a global desire for sustainable chemistry has led to the resurgence of …

Photoredox catalysis via consecutive 2 LMCT-and 3 MLCT-excitation of an Fe (iii/ii)–N-heterocyclic carbene complex

A Ilic, J Schwarz, C Johnson, LHM de Groot… - Chemical …, 2022 - pubs.rsc.org
Fe–N-heterocyclic carbene (NHC) complexes attract increasing attention as
photosensitisers and photoredox catalysts. Such applications generally rely on sufficiently …

Ferrous and ferric complexes with cyclometalating N-heterocyclic carbene ligands: a case of dual emission revisited

CE Johnson, J Schwarz, M Deegbey, O Prakash… - Chemical …, 2023 - pubs.rsc.org
Iron N-heterocyclic carbene (FeNHC) complexes with long-lived charge transfer states are
emerging as a promising class of photoactive materials. We have synthesized [FeII (ImP) …

Electronic Structures and Photoredox Chemistry of Tungsten (0) Arylisocyanides

AT Barth, J Fajardo Jr, W Sattler… - Accounts of Chemical …, 2023 - ACS Publications
Conspectus The high energy barriers associated with the reaction chemistry of inert
substrates can be overcome by employing redox-active photocatalysts. Research in this …

Factors that Impact Photochemical Cage Escape Yields

MJ Goodwin, JC Dickenson, A Ripak, AM Deetz… - Chemical …, 2024 - ACS Publications
The utilization of visible light to mediate chemical reactions in fluid solutions has
applications that range from solar fuel production to medicine and organic synthesis. These …

Spectroscopic Techniques to Unravel Mechanistic Details in Light‐Induced Transformations and Photoredox Catalysis

S De Kreijger, M Gillard, B Elias… - …, 2024 - Wiley Online Library
The rapid development of photo (redox) catalysis within the last decades is remarkable to
the extent that the utilization of light‐driven processes in organic chemistry has become a …

[HTML][HTML] A protocol for determining cage-escape yields using nanosecond transient absorption spectroscopy

A Ripak, S De Kreijger, B Elias, L Troian-Gautier - STAR protocols, 2023 - Elsevier
Here, we present a protocol for the determination of cage-escape yields following excited-
state electron transfer between a photosensitizer and a quencher. We describe steps for …

Investigation of the Excited-State Electron Transfer and Cage Escape Yields Between Halides and a Fe (III) Photosensitizer

S De Kreijger, A Ripak, B Elias… - Journal of the American …, 2024 - ACS Publications
Excited-state quenching and reduction of [Fe (phtmeimb) 2]+, where phtmeimb is phenyl [tris
(3-methyl-imidazolin-2-ylidene)] borate, with iodide, bromide, and chloride were studied in …

Competing dynamics of intramolecular deactivation and bimolecular charge transfer processes in luminescent Fe (III) N-heterocyclic carbene complexes

NW Rosemann, L Lindh, IB Losada, S Kaufhold… - Chemical …, 2023 - pubs.rsc.org
Steady state and ultrafast spectroscopy on [FeIII (phtmeimb) 2] PF6 (phtmeimb= phenyl (tris
(3-methylimidazol-2-ylidene)) borate) was performed over a broad range of temperatures …