TURBOMOLE is a highly optimized software suite for large-scale quantum-chemical and
materials science simulations of molecules, clusters, extended systems, and periodic solids …

Molecular magnetism, though distinctly a field within chemistry, encompasses much more
than synthesis and has strong links with other disciplines across the physical sciences …

The thermostable four-coordinate divalent lanthanide (Ln) bis-amidinate complexes [Ln
(Piso) 2](Ln= Tb, Dy; Piso={(NDipp) 2CtBu}, Dipp= C6H3iPr2-2, 6) were prepared by the …

One goal of the second quantum revolution is developing an approach to transmit coherent
quantum information across the world, forming the basis of the quantum Internet. Achieving …

A small but growing number of molecular compounds have been isolated featuring divalent
lanthanides with 4f n 5d z 21 electron configurations. While the majority of these possess …

Optically addressable spins are a promising platform for quantum information science due to
their combination of a long-lived qubit with a spin-optical interface for external qubit control …

Crystal field (CF) control of rare-earth (RE) ions has been employed to minimize
decoherence in qubits and to enhance the effective barrier of single-molecule magnets. The …

The quest for developing quantum technologies is driven by the promise of exponentially
faster computations, ultrahigh performance sensing, and achieving thorough understanding …

We report a supramolecule that contains five spins of two different types and with, crucially,
two different and predictable interaction energies between the spins. The supramolecule is …

Molecular qubits offer an attractive basis for quantum information processing, but challenges
remain with regard to sustained coherence. Qubits based on clock transitions offer a method …