C–H activation

T Rogge, N Kaplaneris, N Chatani, J Kim… - Nature Reviews …, 2021 - nature.com
Transition metal-catalysed C–H activation has emerged as an increasingly powerful platform
for molecular syntheses, enabling applications to natural product syntheses, late-stage …

Late‐stage peptide diversification by position‐selective C− H activation

W Wang, MM Lorion, J Shah, AR Kapdi… - Angewandte Chemie …, 2018 - Wiley Online Library
The late‐stage modification of structurally complex peptides bears great potential for drug
discovery, crop protection, and the pharmaceutical industry, among others. Whereas …

Manganese‐Catalyzed C− H Alkynylation: Expedient Peptide Synthesis and Modification

Z Ruan, N Sauermann, E Manoni… - Angewandte …, 2017 - Wiley Online Library
Abstract Manganese (I)‐catalyzed C− H alkynylations with organic halides occurred with
unparalleled substrate scope, and thus enabled step‐economical C− H functionalizations …

Cyclic hypervalent iodine reagents: enabling tools for bond disconnection via reactivity umpolung

DP Hari, P Caramenti, J Waser - Accounts of chemical research, 2018 - ACS Publications
Conspectus The efficient synthesis of organic compounds is an important field of research,
which sets the basis for numerous applications in medicine or materials science. Based on …

Postassembly modifications of peptides via metal-catalyzed C–H functionalization

HR Tong, B Li, G Li, G He, G Chen - CCS Chemistry, 2021 - chinesechemsoc.org
The growing importance of peptides and proteins in therapeutic and biomedical applications
has provided immense motivation toward the development of new ways to construct and …

Progress and perspectives on directing group-assisted palladium-catalysed C–H functionalisation of amino acids and peptides

S Shabani, Y Wu, HG Ryan, CA Hutton - Chemical Society Reviews, 2021 - pubs.rsc.org
Peptide modifications can unlock a variety of compounds with structural diversity and
abundant biological activity. In nature, peptide modifications, such as functionalisation at the …

C‐Terminal Bioconjugation of Peptides through Photoredox Catalyzed Decarboxylative Alkynylation

M Garreau, F Le Vaillant, J Waser - Angewandte Chemie …, 2019 - Wiley Online Library
We report the first decarboxylative alkynylation of the C‐terminus of peptides starting from
free carboxylic acids. The reaction is fast, metal‐free, and proceeds cleanly to afford …

Gold and hypervalent iodine (III): liaisons over a decade for electrophilic functional group transfer reactions

S Banerjee, VW Bhoyare, NT Patil - Chemical Communications, 2020 - pubs.rsc.org
Over the last two decades, hypervalent iodine (III) reagents have evolved from being
'bonding curiosities' to mainstream reagents in organic synthesis, in particular, electrophilic …

Late‐Stage Peptide Diversification through Cobalt‐Catalyzed C− H Activation: Sequential Multicatalysis for Stapled Peptides

MM Lorion, N Kaplaneris, J Son, R Kuniyil… - Angewandte …, 2019 - Wiley Online Library
Bioorthogonal late‐stage diversification of structurally complex peptides has enormous
potential for drug discovery and molecular imaging. In recent years, transition‐metal …

BODIPY Peptide Labeling by Late‐Stage C(sp3)−H Activation

W Wang, MM Lorion, O Martinazzoli… - Angewandte Chemie …, 2018 - Wiley Online Library
Late‐stage BODIPY diversification of structurally complex amino acids and peptides was
accomplished by racemization‐free palladium‐catalyzed C (sp3)− H activation …