[HTML][HTML] Excess-entropy scaling in supercooled binary mixtures
Transport coefficients, such as viscosity or diffusion coefficient, show significant dependence
on density or temperature near the glass transition. Although several theories have been …
on density or temperature near the glass transition. Although several theories have been …
Polymer glass formation: Role of activation free energy, configurational entropy, and collective motion
WS Xu, JF Douglas, ZY Sun - Macromolecules, 2021 - ACS Publications
We provide a perspective on polymer glass formation, with an emphasis on models in which
the fluid entropy and collective particle motion dominate the theoretical description and data …
the fluid entropy and collective particle motion dominate the theoretical description and data …
Rethinking Mean-Field Glassy Dynamics and Its Relation with the Energy Landscape: The Surprising Case of the Spherical Mixed -Spin Model
The spherical p-spin model is a fundamental model in statistical mechanics of a disordered
system with a random first-order transition. The dynamics of this model is interesting both for …
system with a random first-order transition. The dynamics of this model is interesting both for …
[HTML][HTML] Dynamic heterogeneity, cooperative motion, and Johari–Goldstein -relaxation in a metallic glass-forming material exhibiting a fragile-to-strong transition
Abstract We investigate the Johari–Goldstein (JG) β β-relaxation process in a model metallic
glass-forming (GF) material (Al _ 90 Sm _ 10 Al 90 Sm 10), previously studied extensively by …
glass-forming (GF) material (Al _ 90 Sm _ 10 Al 90 Sm 10), previously studied extensively by …
Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function
We compare glassy dynamics in two liquids that differ in the form of their interaction
potentials. Both systems have the same repulsive interactions but one has also an attractive …
potentials. Both systems have the same repulsive interactions but one has also an attractive …
A comparative study of the correlation between the structure and the dynamics for systems interacting via attractive and repulsive potentials
We present the study of the structure–dynamics correlation for systems interacting via
attractive Lennard-Jones (LJ) and its repulsive counterpart, the Weeks–Chandler–Andersen …
attractive Lennard-Jones (LJ) and its repulsive counterpart, the Weeks–Chandler–Andersen …
Microscopic theory of softness in supercooled liquids
MK Nandi, SM Bhattacharyya - Physical Review Letters, 2021 - APS
We introduce a new measure of the structure of a liquid which is the softness of the mean-
field potential developed by us earlier. We find that this softness is sensitive to small …
field potential developed by us earlier. We find that this softness is sensitive to small …
[HTML][HTML] Diffusion in dense supercritical methane from quasi-elastic neutron scattering measurements
U Ranieri, S Klotz, R Gaal, MM Koza… - Nature communications, 2021 - nature.com
Methane, the principal component of natural gas, is an important energy source and raw
material for chemical reactions. It also plays a significant role in planetary physics, being one …
material for chemical reactions. It also plays a significant role in planetary physics, being one …
Mechanical disorder of sticky-sphere glasses. II. Thermomechanical inannealability
Many structural glasses feature static and dynamic mechanical properties that can depend
strongly on glass formation history. The degree of universality of this history dependence …
strongly on glass formation history. The degree of universality of this history dependence …
Role of attractive forces in the relaxation dynamics of supercooled liquids
J Chattoraj, MP Ciamarra - Physical Review Letters, 2020 - APS
The attractive tail of the intermolecular interaction affects very weakly the structural
properties of liquids, while it affects dramatically their dynamical ones. Via the numerical …
properties of liquids, while it affects dramatically their dynamical ones. Via the numerical …