Molecular main group metal hydrides

MMD Roy, AA Omana, ASS Wilson, MS Hill… - Chemical …, 2021 - ACS Publications
This review serves to document advances in the synthesis, versatile bonding, and reactivity
of molecular main group metal hydrides within Groups 1, 2, and 12–16. Particular attention …

Combining chemistry and protein engineering for new-to-nature biocatalysis

DC Miller, SV Athavale, FH Arnold - Nature Synthesis, 2022 - nature.com
Biocatalysis, the application of enzymes to solve synthetic problems of human import, has
blossomed into a powerful technology for chemical innovation. In the past decade, a …

Reactions of hydrosilanes with transition metal complexes

JY Corey - Chemical Reviews, 2016 - ACS Publications
This third review in a series involving reactions of hydrosilanes and transition metal
complexes and characterization of the products covers the period 2009 thru 2013. After a …

Accessing zinc monohydride cations through coordinative interactions

PA Lummis, MR Momeni, MW Lui… - Angewandte …, 2014 - Wiley Online Library
We present isolable examples of formal zinc hydride cations supported by N‐heterocyclic
carbene (NHC) donors, and investigate the dual electrophilic and nucleophilic (hydridic) …

Zinc hydride-catalyzed hydrofuntionalization of ketones

RK Sahoo, M Mahato, A Jana… - The Journal of Organic …, 2020 - ACS Publications
Three new dimeric bis-guanidinate zinc (II) alkyl, halide, and hydride complexes [LZnEt] 2
(1),[LZnI] 2 (2) and [LZnH] 2 (3) were prepared. Compound 3 was successfully employed for …

Abiotic reduction of ketones with silanes catalysed by carbonic anhydrase through an enzymatic zinc hydride

P Ji, J Park, Y Gu, DS Clark, JF Hartwig - Nature chemistry, 2021 - nature.com
Enzymatic reactions through mononuclear metal hydrides are unknown in nature, despite
the prevalence of such intermediates in the reactions of synthetic transition-metal catalysts. If …

A Cationic Zinc Hydride Cluster Stabilized by an N‐Heterocyclic Carbene: Synthesis, Reactivity, and Hydrosilylation Catalysis

A Rit, A Zanardi, TP Spaniol, L Maron… - Angewandte Chemie …, 2014 - Wiley Online Library
The trinuclear cationic zinc hydride cluster [(IMes) 3Zn3H4 (THF)](BPh4) 2 (1) was obtained
either by protonation of the neutral zinc dihydride [(IMes) ZnH2] 2 with a Brønsted acid or by …

Synthesis, Structure, and Reactivity of a Mononuclear Organozinc Hydride Complex: Facile Insertion of CO2 into a Zn–H Bond and CO2-Promoted Displacement of …

W Sattler, G Parkin - Journal of the American Chemical Society, 2011 - ACS Publications
Tris (2-pyridylthio) methane,[Tptm] H, has been employed to synthesize the mononuclear
alkyl zinc hydride complex,[κ3-Tptm] ZnH, which has been structurally characterized by X …

H2 Cleavage, Hydride Formation, and Catalytic Hydrogenation of Imines with Zinc Complexes of C5Me5 and N-Heterocyclic Carbenes.

P Jochmann, DW Stephan - … Chemie International Edition, 2013 - search.ebscohost.com
The article presents a study which aims to investigates the reactivity of decamethylzincocene
with various N-heterocyclic carbenes (NHCs) that yields an adduct or a sterically Lewis pair …

Coordinatively saturated tris (oxazolinyl) borato zinc hydride-catalyzed cross dehydrocoupling of silanes and alcohols

D Mukherjee, RR Thompson, A Ellern, AD Sadow - ACS Catalysis, 2011 - ACS Publications
The four-coordinate zinc compound ToMZnH (1, ToM= tris (4, 4-dimethyl-2-oxazolinyl)
phenylborate) catalyzes selective alcoholysis of substituted hydrosilanes. The catalytic …