The fracture of highly deformable soft materials: A tale of two length scales

R Long, CY Hui, JP Gong… - Annual Review of …, 2021 - annualreviews.org
The fracture of highly deformable soft materials is of great practical importance in a wide
range of technological applications, emerging in fields such as soft robotics, stretchable …

Crack tip field of a double-network gel: Visualization of covalent bond scission through mechanoradical polymerization

T Matsuda, R Kawakami, T Nakajima, JP Gong - Macromolecules, 2020 - ACS Publications
Quantitative characterization of the energy dissipation zone around a crack tip is the focal
point in the fracture mechanics of soft materials. In this report, we present a …

A molecular interpretation of the toughness of multiple network elastomers at high temperature

J Slootman, CJ Yeh, P Millereau… - Proceedings of the …, 2022 - National Acad Sciences
Unfilled elastomers often suffer from poor fracture resistance at high temperature where
viscoelastic dissipation is low. A molecular design based on multiple interpenetrating …

Unique crack propagation of double network hydrogels under high stretch

Y Zhang, K Fukao, T Matsuda, T Nakajima… - Extreme Mechanics …, 2022 - Elsevier
Double network (DN) gels, consisting of two contrasting interpenetrated polymer networks,
exhibit large resistances to crack initiation and propagation. For practical applications, crack …

Material perspective on the structural design of artificial meat

J He, Y Zhao, X Jin, X Zhu… - Advanced Sustainable …, 2021 - Wiley Online Library
Artificial meat is a promising solution to the negative impacts of meat consumption on natural
resources, public health, and animal welfare. Inspired by the use of framework, scaffold, and …

How chain dynamics affects crack initiation in double-network gels

Y Zheng, T Matsuda, T Nakajima… - Proceedings of the …, 2021 - National Acad Sciences
Double-network gels are a class of tough soft materials comprising two elastic networks with
contrasting structures. The formation of a large internal damage zone ahead of the crack tip …

[HTML][HTML] Crack tip kinematics reveal the process zone structure in brittle hydrogel fracture

C Li, X Wei, M Wang, M Adda-Bedia… - Journal of the Mechanics …, 2023 - Elsevier
When brittle hydrogels fail, several mechanisms conspire to alter the state of stress near the
tip of a crack, and it is challenging to identify which mechanism is dominant. In the fracture of …

Effect of predamage on the fracture energy of double-network hydrogels

Y Zheng, Y Wang, T Nakajima, JP Gong - ACS Macro Letters, 2024 - ACS Publications
Double-network (DN) hydrogels are tough soft materials, and the high fracture resistance
can be attributed to the formation of a large damage zone (internal fracture of the brittle first …

Real-Time Early Detection of Crack Propagation Precursors in Delayed Fracture of Soft Elastomers

J Ju, GE Sanoja, MY Nagazi, L Cipelletti, Z Liu, CY Hui… - Physical Review X, 2023 - APS
The fracture of materials can take place below the critical failure condition via the slow
accumulation of internal damage followed by fast crack propagation. While failure due to …

Dynamic responses of Ca-alginate/polyacrylamide hydrogels at high strain rates

Q Xue, Y Xiao, X Zhang, X Zhang, W Hong… - International Journal of …, 2024 - Elsevier
Many biological hydrogels possess remarkable mechanical performances under both quasi-
static and impact loadings, yet such mechanical robustness over a wide range of strain rates …