Molecular views on Fischer–Tropsch synthesis

KT Rommens, M Saeys - Chemical Reviews, 2023 - ACS Publications
For nearly a century, the Fischer–Tropsch (FT) reaction has been subject of intense debate.
Various molecular views on the active sites and on the reaction mechanism have been …

Recent advances on syngas conversion targeting light olefins

S Zhao, H Li, B Wang, X Yang, Y Peng, H Du, Y Zhang… - Fuel, 2022 - Elsevier
The direct synthesis of light olefins (C 2 H 4, C 3 H 6 and C 4 H 8) from syngas (a mixture of
H 2 and CO) could supply the extra resources of these platform building blocks for the …

Advances in selectivity control for Fischer–Tropsch synthesis to fuels and chemicals with high carbon efficiency

T Lin, Y An, F Yu, K Gong, H Yu, C Wang, Y Sun… - ACS …, 2022 - ACS Publications
Fischer–Tropsch synthesis (FTS) is a versatile technology to produce high-quality fuels and
key building-block chemicals from syngas derived from nonpetroleum carbon resources …

Cobalt carbide nanocatalysts for efficient syngas conversion to value-added chemicals with high selectivity

T Lin, F Yu, Y An, T Qin, L Li, K Gong… - Accounts of Chemical …, 2021 - ACS Publications
Conspectus Syngas conversion is a key platform for efficient utilization of various carbon-
containing resources including coal, natural gas, biomass, organic wastes, and even CO2 …

The oscillating fischer-tropsch reaction

R Zhang, Y Wang, P Gaspard, N Kruse - Science, 2023 - science.org
The mechanistic steps that underlie the formation of higher hydrocarbons in catalytic carbon
monoxide (CO) hydrogenation at atmospheric pressure over cobalt-based catalysts (Fischer …

The active phase in cobalt-based Fischer-Tropsch synthesis

IC ten Have, BM Weckhuysen - Chem Catalysis, 2021 - cell.com
Fischer-Tropsch synthesis (FTS) is an industrial catalytic process that converts a mixture of
CO and hydrogen into long-chain hydrocarbons. These products are used as clean …

Regulating oxygen vacancies for enhanced higher oxygenate synthesis via syngas

X Qi, T Lin, Y An, X Wang, D Lv, Z Tang, L Zhong - ACS Catalysis, 2023 - ACS Publications
Constructing highly efficient dual active sites for preferential formation of higher oxygenates
via direct syngas conversion remains a grand challenge. Herein, we reported that the …

Recent advances in application of iron-based catalysts for COx hydrogenation to value-added hydrocarbons

J Liu, Y Song, X Guo, C Song, X Guo - Chinese Journal of Catalysis, 2022 - Elsevier
The widespread utilization of fossil fuels has caused an associated increase in CO 2
emissions over the past few decades, which has resulted in global warming and ocean …

Fischer–Tropsch Synthesis to Olefins: Catalytic Performance and Structure Evolution of Co2C-Based Catalysts under a CO2 Environment

T Lin, K Gong, C Wang, Y An, X Wang, X Qi, S Li… - ACS …, 2019 - ACS Publications
Cobalt carbide (Co2C) nanoprisms derived from CoMn composite oxides exhibit promising
catalytic performance for Fischer–Tropsch to olefins (FTO) synthesis via H2-lean syngas …

Morphological Modulation of Co2C by Surface-Adsorbed Species for Highly Effective Low-Temperature CO2 Reduction

S Zhang, X Liu, H Luo, Z Wu, B Wei, Z Shao… - ACS …, 2022 - ACS Publications
Modulating the morphologies of transition metal carbides (TMCs) in situ in gas–solid
reactions to improve catalytic performance remains a major challenge. Herein, we present a …